Recombination dynamics of luminescence in colloidal CdSe/ZrS quantum dots

被引:55
作者
Lee, WZ
Shu, GW
Wang, JS
Shen, JL [1 ]
Lin, CA
Chang, WH
Ruaan, RC
Chou, WC
Lu, CH
Lee, YC
机构
[1] Chung Yuan Christian Univ, Dept Phys, Chungli, Taiwan
[2] Chung Yuan Christian Univ, Dept Biomed Engn, Chungli, Taiwan
[3] Natl Cent Univ, Dept Chem & Mat Engn, Chungli 32054, Taiwan
[4] Natl Chiao Tung Univ, Electrophys Dept, Hsinchu, Taiwan
[5] Natl Taiwan Univ, Dept Chem Engn, Taipei 10764, Taiwan
[6] Tung Nan Inst Technol, Dept Comp Sci & Informat Engn, Taipei, Taiwan
关键词
D O I
10.1088/0957-4484/16/9/018
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Recombination dynamics of photoluminescence (PL) in colloidal CdSe/ZnS quantum dots (QDs) were studied using time-resolved PL measurements. The PL intensity shows a biexponential decay at 9 K, consisting of a fast component (similar to 1 ns) and a slow component (similar to 6.3 ns). Based on the emission-energy and temperature dependence of carrier lifetimes, we suggest that the fast and slow PL decay of colloidal CdSe/ZnS QDs originates from recombination of the delocalized carriers in the internal core states and the localized carriers at the interface, respectively.
引用
收藏
页码:1517 / 1521
页数:5
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