Interplay between orbital and magnetic long range order by resonant X-ray scattering in (V1-xCrx)2O3

被引:32
作者
Paolasini, L
Di Matteo, S
Vettier, C
de Bergevin, F
Sollier, A
Neubeck, W
Yakhou, F
Metcalf, PA
Honig, JM
机构
[1] European Synchrotron Radiat Facil, F-38043 Grenoble 9, France
[2] Inst Max Von Laue Paul Langevin, F-38042 Grenoble 9, France
[3] Purdue Univ, Dept Chem, W Lafayette, IN 47907 USA
[4] Univ Salerno, Dipartimento Sci Fis, I-84081 Baronissi, Salerno, Italy
关键词
vanadium sesquioxide; orbital ordering; resonant X-ray scattering;
D O I
10.1016/S0368-2048(01)00307-3
中图分类号
O433 [光谱学];
学科分类号
0703 ; 070302 ;
摘要
Resonant X-ray scattering experiments have been performed in 2.8% Cr-doped V2O3 single crystal at the Vanadium K-photoabsorption edge. Using linear polarization analysis and comparing the angular dependence of scattered photons with structure factor calculations we can discriminate the nature of the different resonant X-ray processes involved in forbidden lattice reflections enhanced by resonances. We present an experimental method to extract information on local properties of edge-atom such as the anisotropy of the local atomic environment, the atomic magnetic moment orientation and orbital ordering. (C) 2001 Elsevier Science BM All rights reserved.
引用
收藏
页码:1 / 10
页数:10
相关论文
共 33 条
[11]   Orbital occupation, local spin, and exchange interactions in V2O3 [J].
Ezhov, SY ;
Anisimov, VI ;
Khomskii, DI ;
Sawatzky, GA .
PHYSICAL REVIEW LETTERS, 1999, 83 (20) :4136-4139
[12]   X-ray resonant scattering as a direct probe of orbital ordering in transition-metal oxides [J].
Fabrizio, M ;
Altarelli, M ;
Benfatto, M .
PHYSICAL REVIEW LETTERS, 1998, 80 (15) :3400-3403
[13]  
FABRIZIO M, COMMUNICATION
[14]   RESONANT X-RAY-DIFFRACTION NEAR THE IRON-K EDGE IN HEMATITE (ALPHA-FE2O3) [J].
FINKELSTEIN, KD ;
SHEN, Q ;
SHASTRI, S .
PHYSICAL REVIEW LETTERS, 1992, 69 (10) :1612-1615
[15]   X-RAY RESONANCE EXCHANGE SCATTERING [J].
HANNON, JP ;
TRAMMELL, GT ;
BLUME, M ;
GIBBS, D .
PHYSICAL REVIEW LETTERS, 1988, 61 (10) :1245-1248
[16]   X-ray resonant exchange scattering: Polarization dependence and correlation functions [J].
Hill, JP ;
McMorrow, DF .
ACTA CRYSTALLOGRAPHICA SECTION A, 1996, 52 (02) :236-244
[17]   Metal-insulator transitions [J].
Imada, M ;
Fujimori, A ;
Tokura, Y .
REVIEWS OF MODERN PHYSICS, 1998, 70 (04) :1039-1263
[18]   ANISOTROPY OF ANOMALOUS SCATTERING IN X-RAY-DIFFRACTION .2. COMBINING POLARIZATION-DEPENDENT TRANSMISSION AND DIFFRACTION, AND AN APPLICATION TO PARTIAL-STRUCTURE ANALYSIS [J].
KIRFEL, A ;
PETCOV, A .
ACTA CRYSTALLOGRAPHICA SECTION A, 1992, 48 :247-259
[19]   Resonant x-ray Bragg diffraction from orbital moments in vanadium sesquioxide (V2O3) and haematite (α -Fe2O3) [J].
Lovesey, SW ;
Knight, KS .
JOURNAL OF PHYSICS-CONDENSED MATTER, 2000, 12 (23) :L367-L372
[20]   Metal-insulator transition in (V1-xCrx)(2)O-3 [J].
McWhan, D. B. ;
Remeika, J. P. .
PHYSICAL REVIEW B-SOLID STATE, 1970, 2 (09) :3734-3750