A high-resolution ammonia emission inventory in China

被引：423

作者：

Huang, Xin ^{[1
]}

Song, Yu ^{[1
]}

Li, Mengmeng ^{[1
]}

Li, Jianfeng ^{[1
]}

Huo, Qing ^{[1
]}

Cai, Xuhui ^{[1
]}

Zhu, Tong ^{[1
]}

Hu, Min ^{[1
]}

Zhang, Hongsheng ^{[2
]}

机构：

[1] Peking Univ, Dept Environm Sci, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100871, Peoples R China

[2] Peking Univ, Sch Phys, Dept Atmospher & Ocean Sci, Lab Atmosphere Ocean Studies, Beijing 100871, Peoples R China

来源：

GLOBAL BIOGEOCHEMICAL CYCLES | 2012年 / 26卷

基金：

中国国家自然科学基金;

关键词：

ATMOSPHERIC AMMONIA; NITROGEN LOSS; VOLATILIZATION LOSSES; NH3; EMISSIONS; EAST-ASIA; FERTILIZERS; UREA; LIVESTOCK; MODEL; RICE;

D O I：

10.1029/2011GB004161

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

The existence of gas-phase ammonia (NH3) in the atmosphere and its interaction with other trace chemical species could have a substantial impact on tropospheric chemistry and global climate change. China is a large agricultural country with an enormous animal population, tremendous nitrogen fertilizer consumption and, consequently, a large emission of NH3. Despite the importance of NH3 in the global nitrogen (N) cycle, considerable inaccuracies and uncertainty exist regarding its emission in China. In this study, a comprehensive NH3 emission inventory was compiled for China on a 1 km x 1 km grid, which is suitable for input to atmospheric models. We attempted to estimate NH3 emissions accurately by taking into consideration as many native experiment results as possible and parameterizing the emission factors (EFs) by the ambient temperature, soil acidity and other factors. The total NH3 emission in China was approximately 9.8 Tg in 2006. The emission sources considered included livestock excreta (5.3 Tg), fertilizer application (3.2 Tg), agricultural soil (0.2 Tg), nitrogen-fixing plants (0.05 Tg), crop residue compost (0.3 Tg), biomass burning (0.1 Tg), urine from rural populations (0.2 Tg), chemical industry (0.2 Tg), waste disposal (0.1 Tg) and traffic (0.1 Tg). The regions with the highest emission rates are located in Central and Southwest China. Seasonally, the peak ammonia emissions occur in spring and summer.

引用

页数：14

共 95 条

[41] World crop residues production and implications of its use as a biofuel [J].

Lal, R .

ENVIRONMENT INTERNATIONAL, 2005, 31 (04) :575-584

[42]

[李贵桐 Li Guitong], 2002, [华北农学报, Acta Agriculturae Boreali-Sinica], V17, P76

[43]

[李剑睿 LI Jian-rui], 2009, [农业环境科学学报, Journal of Agro-Environment Science], V28, P1959

[44]

Li S., 1993, AGR RES ARID AREAS, V11, P130

[45] Particulate and trace gas emissions from open burning of wheat straw and corn stover in China [J].

Li, Xinghua ;

Wang, Shuxiao ;

Duan, Lei ;

Hao, Jiming ;

Li, Chao ;

Chen, Yaosheng ;

Yang, Liu .

ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2007, 41 (17) :6052-6058

[46] Long-range transport of acidifying substances in East Asia - Part I - Model evaluation and sensitivity studies [J].

Lin, Meiyun ;

Oki, Taikan ;

Holloway, Tracey ;

Streets, David G. ;

Bengtsson, Magnus ;

Kanae, Shinjiro .

ATMOSPHERIC ENVIRONMENT, 2008, 42 (24) :5939-5955

[47]

Liu Dong Liu Dong, 2008, Transactions of the Chinese Society of Agricultural Engineering, V24, P218

[48]

Lu D., 1980, SHAANXI J AGR SCI, V6, P7

[49]

Mannebeck H., 1991, Odour and ammonia emissions from livestock farming. Proceedings of a seminar, Silsoe, UK, 26-28 March l990.., P42

[50] Effects of the physical state of tropospheric ammonium-sulfate-nitrate particles on global aerosol direct radiative forcing [J].

Martin, ST ;

Hung, HM ;

Park, RJ ;

Jacob, DJ ;

Spurr, RJD ;

Chance, KV ;

Chin, M .

ATMOSPHERIC CHEMISTRY AND PHYSICS, 2004, 4 :183-214

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