Recent developments of molybdenum and tungsten sulfides as hydrogen evolution catalysts

被引:1092
作者
Merki, Daniel [1 ]
Hu, Xile [1 ]
机构
[1] Ecole Polytech Fed Lausanne EPFL, Lab Inorgan Synth & Catalysis, Inst Chem Sci & Engn, EPFL ISIC LSCI, CH-1015 Lausanne, Switzerland
基金
欧洲研究理事会;
关键词
ATOMIC-SCALE STRUCTURE; MOS2; THIN-FILMS; ELECTROCHEMICAL DEPOSITION; S NANOCLUSTERS; H-2; EVOLUTION; ELECTROCATALYSTS; MORPHOLOGY; DISULFIDE;
D O I
10.1039/c1ee01970h
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Recent work shows that nanoparticulate and amorphous molybdenum and tungsten sulfide materials are active catalysts for hydrogen evolution in aqueous solution. These materials hold promise for applications in clean hydrogen production technologies. In this perspective, the syntheses, structures and catalytic activities of nanoparticulate MoS2 and WS2, incomplete cubane-type [Mo3S4](4+) and amorphous MoSx films are summarized, compared, and discussed.
引用
收藏
页码:3878 / 3888
页数:11
相关论文
共 49 条
[1]   GROWTH OF TUNGSTENITE SINGLE-CRYSTALS BY DIRECT VAPOR TRANSPORT METHOD [J].
AGARWAL, MK ;
NAGIREDDY, K ;
PATEL, HB .
JOURNAL OF CRYSTAL GROWTH, 1979, 46 (01) :139-142
[2]   A NICKEL MOLYBDENITE CATHODE FOR THE HYDROGEN EVOLUTION REACTION IN ALKALINE MEDIA [J].
ALBERTINI, LB ;
ANGELO, ACD ;
GONZALEZ, ER .
JOURNAL OF APPLIED ELECTROCHEMISTRY, 1992, 22 (09) :888-892
[3]   A study on MoS2 thin films electrochemically deposited in ethylene glycol at 165°C [J].
Albu-Yaron, A ;
Levy-Clement, C ;
Hutchison, JL .
ELECTROCHEMICAL AND SOLID STATE LETTERS, 1999, 2 (12) :627-630
[4]   Molybdenum-sulfur dimers as electrocatalysts for the production of hydrogen at low overpotentials [J].
Appel, AM ;
DuBois, DL ;
DuBois, MR .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2005, 127 (36) :12717-12726
[5]   Some general principles for designing electrocatalysts with hydrogenase activity [J].
Artero, V ;
Fontecave, M .
COORDINATION CHEMISTRY REVIEWS, 2005, 249 (15-16) :1518-1535
[6]   THE ELECTRODEPOSITION OF AMORPHOUS MOLYBDENUM SULFIDE [J].
BELANGER, D ;
LAPERRIERE, G ;
MARSAN, B .
JOURNAL OF ELECTROANALYTICAL CHEMISTRY, 1993, 347 (1-2) :165-183
[7]   THE MECHANISM OF THE CATHODIC HYDROGEN EVOLUTION REACTION [J].
BOCKRIS, JOM ;
POTTER, EC .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 1952, 99 (04) :169-186
[8]   Energy-Conversion Properties of Vapor-Liquid-Solid-Grown Silicon Wire-Array Photocathodes [J].
Boettcher, Shannon W. ;
Spurgeon, Joshua M. ;
Putnam, Morgan C. ;
Warren, Emily L. ;
Turner-Evans, Daniel B. ;
Kelzenberg, Michael D. ;
Maiolo, James R. ;
Atwater, Harry A. ;
Lewis, Nathan S. .
SCIENCE, 2010, 327 (5962) :185-187
[9]   Hydrogen evolution on nano-particulate transition metal sulfides [J].
Bonde, Jacob ;
Moses, Poul G. ;
Jaramillo, Thomas F. ;
Norskov, Jens K. ;
Chorkendorff, Ib .
FARADAY DISCUSSIONS, 2008, 140 :219-231
[10]   The morphology of MoS2, WS2, Co-Mo-S, Ni-Mo-S and Ni-W-S nanoclusters in hydrodesulfurization catalysts revealed [J].
Brorson, M. ;
Carlsson, A. ;
Topsoe, H. .
CATALYSIS TODAY, 2007, 123 (1-4) :31-36