Influence of residential wood combustion on local air quality

被引:81
作者
Hellen, H. [1 ]
Hakola, H. [1 ]
Haaparanta, S. [1 ]
Pietarila, H. [1 ]
Kauhaniemi, M. [1 ]
机构
[1] Finnish Meteorol Inst, FIN-00101 Helsinki, Finland
关键词
wood combustion; air quality; VOCs; PAHs; CMB;
D O I
10.1016/j.scitotenv.2008.01.019
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The importance of wood combustion to local air quality was estimated by measuring different air pollutants and conducting chemical mass balance modelling. PM10, PM2.5, PAHs and VOC concentrations in ambient air were measured in a typical Finnish residential area. Measurements were conducted in January-March 2006. For some compounds, wood combustion was clearly the main local source at this site. The effect of wood combustion was more clearly seen for organic compounds than for fine particle mass. For fine particles, background concentrations dominated. However, very high, short-lived concentration peaks were detected, when the wind direction and other weather conditions were favourable. For organic compounds, the effect of wood combustion was seen in diurnal and in two-week average concentrations. PAH-concentrations were often several times higher at the residential area than in the background. Benzene concentrations showed similar diurnal pattern as the use of wood and benzene/toluene ratios indicated that wood combustion is the most important source. A chemical mass balance model was used for studying the effect of wood combustion on the measured concentrations of VOCs. Model results showed that the main local sources for VOCs at Kurkimaki are wood combustion and traffic. Wood combustion was clearly the most important source for many compounds (e.g., benzene). (C) 2008 Elsevier B.V. All rights reserved.
引用
收藏
页码:283 / 290
页数:8
相关论文
共 28 条
[11]   Carbonyl compounds in boreal coniferous forest air in Hyytiala, Southern Finland [J].
Hellén, H ;
Hakola, H ;
Reissell, A ;
Ruuskanen, TM .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2004, 4 :1771-1780
[12]   Determination of source contributions of NMHCs in Helsinki (60°N, 25°E) using chemical mass balance and the Unmix multivariate receptor models [J].
Hellén, H ;
Hakola, H ;
Laurila, T .
ATMOSPHERIC ENVIRONMENT, 2003, 37 (11) :1413-1424
[13]   Aromatic hydrocarbon and methyl tert-butyl, ether measurements in ambient air of Helsinki (Finland) using diffusive samplers [J].
Hellén, H ;
Hakola, H ;
Laurila, T ;
Hiltunen, V ;
Koskentalo, T .
SCIENCE OF THE TOTAL ENVIRONMENT, 2002, 298 (1-3) :55-64
[14]  
HOPKE PK, 1991, DATA HANDLING SCI TE, V7
[15]  
*ISO, 2000, 10473 ISO
[16]   Emission characteristics of modern and old-type residential boilers fired with wood logs and wood pellets [J].
Johansson, LS ;
Leckner, B ;
Gustavsson, L ;
Cooper, D ;
Tullin, C ;
Potter, A .
ATMOSPHERIC ENVIRONMENT, 2004, 38 (25) :4183-4195
[17]   Effect of airflow setting on the organic composition of woodheater emissions [J].
Jordan, TB ;
Seen, AJ .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2005, 39 (10) :3601-3610
[18]   Receptor modeling of C2-C7 hydrocarbon sources at an urban background site in Zurich, Switzerland:: changes between 1993-1994 and 2005-2006 [J].
Lanz, V. A. ;
Hueglin, C. ;
Buchmann, B. ;
Hill, M. ;
Locher, R. ;
Staehelin, J. ;
Reimann, S. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2008, 8 (09) :2313-2332
[19]   Source apportionment of submicron organic aerosols at an urban site by factor analytical modelling of aerosol mass spectra [J].
Lanz, V. A. ;
Alfarra, M. R. ;
Baltensperger, U. ;
Buchmann, B. ;
Hueglin, C. ;
Prevot, A. S. H. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2007, 7 (06) :1503-1522
[20]   Source apportionment of PM2.5 at an urban IMPROVE site in Seattle, Washington [J].
Maykut, NN ;
Lewtas, J ;
Kim, E ;
Larson, TV .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2003, 37 (22) :5135-5142