Below band-gap nonlinear optical properties of semiconductor-doped glasses

被引:2
作者
Banfi, GP [1 ]
Degiorgio, V [1 ]
Fortusini, D [1 ]
Tan, HM [1 ]
机构
[1] ACAD SINICA, CHANGCHUN INST OPT & FINE MECH, CHANGCHUN, PEOPLES R CHINA
关键词
D O I
10.1142/S0218863596000167
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Through nonlinear transmission and wave-mixing measurements, combined with structural data from neutron scattering, we obtain the below band-gap third-order susceptibility chi((3)) (both imaginary and real part) and the refractive-index-change per carrier of semiconductor nanocrystals embedded in a glass matrix. Our data covers a range of crystal radii between 2 and 14 nm and a range of ratios y = E(g)/(<(h)over bar omega>), where E(g) is the energy gap of the semiconductor and <(h)over bar omega> is the energy of the incident photon, between 1.1 and 1.9. The magnitude of chi((3)) and its dependence on y are comparable to those of related bulk semiconductors.
引用
收藏
页码:205 / 222
页数:18
相关论文
共 32 条
[21]  
PEPPER DM, 1983, OPTICAL PHASE CONJUG
[22]   OPTICAL-ABSORPTION IN SEMICONDUCTOR QUANTUM DOTS - A TIGHT-BINDING APPROACH [J].
RAMANIAH, LM ;
NAIR, SV .
PHYSICAL REVIEW B, 1993, 47 (12) :7132-7139
[23]  
RICARD D, 1995, P INT SCH PHYS, V126, P289
[24]   DETERMINATION OF BOUND-ELECTRONIC AND FREE-CARRIER NONLINEARITIES IN ZNSE, GAAS, CDTE, AND ZNTE [J].
SAID, AA ;
SHEIKBAHAE, M ;
HAGAN, DJ ;
WEI, TH ;
WANG, J ;
YOUNG, J ;
VANSTRYLAND, EW .
JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS, 1992, 9 (03) :405-414
[25]   DISPERSION OF BOUND ELECTRONIC NONLINEAR REFRACTION IN SOLIDS [J].
SHEIKBAHAE, M ;
HUTCHINGS, DC ;
HAGAN, DJ ;
VANSTRYLAND, EW .
IEEE JOURNAL OF QUANTUM ELECTRONICS, 1991, 27 (06) :1296-1309
[26]   DISPERSION AND BAND-GAP SCALING OF THE ELECTRONIC KERR EFFECT IN SOLIDS ASSOCIATED WITH 2-PHOTON ABSORPTION [J].
SHEIKBAHAE, M ;
HAGAN, DJ ;
VANSTRYLAND, EW .
PHYSICAL REVIEW LETTERS, 1990, 65 (01) :96-99
[27]   SIZE DEPENDENCE OF OPTICAL NONLINEARITY OF CDSSE MICROCRYSTALLITES DOPED IN GLASS [J].
SHINOJIMA, H ;
YUMOTO, J ;
UESUGI, N .
APPLIED PHYSICS LETTERS, 1992, 60 (03) :298-300
[28]   2-PHOTON ABSORPTION-COEFFICIENT SPECTRUM IN CDSSE NANOCRYSTALS BY NONLINEAR LUMINESCENCE TECHNIQUE [J].
TOMMASI, R ;
LEPORE, M ;
CATALANO, IM .
SOLID STATE COMMUNICATIONS, 1993, 85 (06) :539-543
[29]   ENERGY BAND-GAP DEPENDENCE OF 2-PHOTON ABSORPTION [J].
VANSTRYLAND, EW ;
WOODALL, MA ;
VANHERZEELE, H ;
SOILEAU, MJ .
OPTICS LETTERS, 1985, 10 (10) :490-492
[30]   OBSERVATION OF OPTICAL BISTABILITY IN CDSXSE1-X-DOPED GLASSES WITH 25-PSEC SWITCHING TIME [J].
YUMOTO, J ;
FUKUSHIMA, S ;
KUBODERA, K .
OPTICS LETTERS, 1987, 12 (10) :832-834