Time-resolved photoluminescence study of the stimulated emission in ZnO nanoneedles

被引:73
作者
Kwok, WM
Djurisic, AB
Leung, YH
Chan, WK
Phillips, DL
机构
[1] Univ Hong Kong, Dept Chem, Hong Kong, Hong Kong, Peoples R China
[2] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China
关键词
D O I
10.1063/1.2035871
中图分类号
O59 [应用物理学];
学科分类号
摘要
ZnO nanoneedles were fabricated by thermal evaporation of Zn nanoparticles at 800 degrees C and atmospheric pressure. The samples showed strong ultraviolet photoluminescence and weak orange defect luminescence. Time-resolved photoluminescence (TRPL) was measured using the Kerr-gated fluorescence technique in order to probe the ultrafast carrier dynamics in exciton-exciton scattering and electron hole plasma (EHP) regimes. In both regimes, the decay time of the photoluminescence is very fast (similar to 1 ps). Even though no structure is detected in the time-integrated spectra of the EHP emission, the TRPL reveals the coexistence of the excitons and free carriers. Possible reasons for the observed phenomena are discussed. (c) 2005 American Institute of Physics.
引用
收藏
页数:3
相关论文
共 25 条
[1]   Coulomb correlation and band gap renormalization at high carrier densities in quantum wires [J].
Ambigapathy, R ;
BarJoseph, I ;
Oberli, DY ;
Haacke, S ;
Brasil, MJ ;
Reinhardt, F ;
Kapon, E ;
Deveaud, B .
PHYSICAL REVIEW LETTERS, 1997, 78 (18) :3579-3582
[2]   Room temperature excitonic stimulated emission from zinc oxide epilayers grown by plasma-assisted MBE [J].
Bagnall, DM ;
Chen, YF ;
Shen, MY ;
Zhu, Z ;
Goto, T ;
Yao, T .
JOURNAL OF CRYSTAL GROWTH, 1998, 184 :605-609
[3]   Spectroscopic evidence for different laser gain mechanisms in optically pumped ZnCdS/ZnS quantum well structures [J].
Chen, P ;
Nicholls, JE ;
O'Neill, M ;
Stirner, T ;
Hogg, JHC ;
Lunn, B ;
Ashenford, DE .
JOURNAL OF APPLIED PHYSICS, 1998, 84 (10) :5621-5625
[4]   Photoluminescence and electron paramagnetic resonance of ZnO tetrapod structure [J].
Djurisic, AB ;
Choy, WCH ;
Roy, VAL ;
Leung, YH ;
Kwong, CY ;
Cheah, KW ;
Rao, TKG ;
Chan, WK ;
Lui, HT ;
Surya, C .
ADVANCED FUNCTIONAL MATERIALS, 2004, 14 (09) :856-864
[5]   Mott transition from a diluted exciton gas to a dense electron-hole plasma in a single V-shaped quantum wire [J].
Guillet, T ;
Grousson, R ;
Voliotis, V ;
Menant, M ;
Wang, XL ;
Ogura, M .
PHYSICAL REVIEW B, 2003, 67 (23)
[6]   Stimulated emission and lasing of random-growth oriented ZnO nanowires [J].
Hsu, HC ;
Wu, CY ;
Hsieh, WF .
JOURNAL OF APPLIED PHYSICS, 2005, 97 (06)
[7]   Ultrafast carrier dynamics in single ZnO nanowire and nanoribbon lasers [J].
Johnson, JC ;
Knutsen, KP ;
Yan, HQ ;
Law, M ;
Zhang, YF ;
Yang, PD ;
Saykally, RJ .
NANO LETTERS, 2004, 4 (02) :197-204
[8]   Optical cavity effects in ZnO nanowire lasers and waveguides [J].
Johnson, JC ;
Yan, HQ ;
Yang, PD ;
Saykally, RJ .
JOURNAL OF PHYSICAL CHEMISTRY B, 2003, 107 (34) :8816-8828
[9]   Spontaneous polarization-induced nanohelixes, nanosprings, and nanorings of piezoelectric nanobelts [J].
Kong, XY ;
Wang, ZL .
NANO LETTERS, 2003, 3 (12) :1625-1631
[10]   Time-resolved study of stimulated emission in ZnO tetrapod nanowires [J].
Leung, YH ;
Kwok, WM ;
Djurisic, AB ;
Phillips, DL ;
Chan, WK .
NANOTECHNOLOGY, 2005, 16 (04) :579-582