A setup for ultrafast time-resolved x-ray absorption spectroscopy

被引:88
作者
Saes, M
Bressler, C [1 ]
van Mourik, F
Gawelda, W
Kaiser, M
Chergui, M
Bressler, C [1 ]
Grolimund, D
Abela, R
Glover, TE
Heimann, PA
Schoenlein, RW
Johnson, SL
Lindenberg, AM
Falcone, RW
机构
[1] Univ Lausanne, IPMC BSP, CH-1015 Lausanne, Switzerland
[2] Paul Scherrer Inst, Nucl Energy & Safety Res Dept, CH-5232 Villigen, Switzerland
[3] Swiss Light Source, CH-5232 Villigen, Switzerland
[4] Univ Calif Berkeley, Lawrence Berkeley Lab, Adv Light Source, Div Mat Sci, Berkeley, CA 94720 USA
[5] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA
关键词
D O I
10.1063/1.1633003
中图分类号
TH7 [仪器、仪表];
学科分类号
0804 ; 080401 ; 081102 ;
摘要
We present a setup which allows the measurement of time-resolved x-ray absorption spectra with picosecond temporal resolution on liquid samples at the Advanced Light Source at Lawrence Berkeley National Laboratories. The temporal resolution is limited by the pulse width of the synchrotron source. We characterize the different sources of noise that limit the experiment and present a single-pulse detection scheme. (C) 2004 American Institute of Physics.
引用
收藏
页码:24 / 30
页数:7
相关论文
共 19 条
[1]   Picosecond laser-pump, x-ray probe spectroscopy of GaAs [J].
Adams, BW ;
DeCamp, MF ;
Dufresne, EM ;
Reis, DA .
REVIEW OF SCIENTIFIC INSTRUMENTS, 2002, 73 (12) :4150-4156
[2]   Towards structural dynamics in condensed chemical systems exploiting ultrafast time-resolved x-ray absorption spectroscopy [J].
Bressler, C ;
Saes, M ;
Chergui, M ;
Grolimund, D ;
Abela, R ;
Pattison, P .
JOURNAL OF CHEMICAL PHYSICS, 2002, 116 (07) :2955-2966
[3]   MLCT state structure and dynamics of a copper(I) diimine complex characterized by pump-probe X-ray and laser spectroscopies and DFT calculations [J].
Chen, LX ;
Shaw, GB ;
Novozhilova, I ;
Liu, T ;
Jennings, G ;
Attenkofer, K ;
Meyer, GJ ;
Coppens, P .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2003, 125 (23) :7022-7034
[4]   Capturing a photoexcited molecular structure through time-domain X-ray absorption fine structure [J].
Chen, LX ;
Jäger, WJH ;
Jennings, G ;
Gosztola, DJ ;
Munkholm, A ;
Hessler, JP .
SCIENCE, 2001, 292 (5515) :262-264
[5]   Femtosecond dynamics of excited-state evolution in [Ru(bpy)(3)](2+) [J].
Damrauer, NH ;
Cerullo, G ;
Yeh, A ;
Boussie, TR ;
Shank, CV ;
McCusker, JK .
SCIENCE, 1997, 275 (5296) :54-57
[6]  
DOUHAL A, 2002, FEMTOCHEMISTRY FEMTO
[7]  
GLOVER TE, 2002, BEAMLINE 5 3 1 SPECT
[8]   LARGE-AREA AVALANCHE PHOTODIODES FOR THE DETECTION OF SOFT X-RAYS [J].
GULLIKSON, EM ;
GRAMSCH, E ;
SZAWLOWSKI, M .
APPLIED OPTICS, 1995, 34 (22) :4662-4668
[9]   Ultrafast X-ray diffraction of laser-irradiated crystals [J].
Heimann, PA ;
Lindenberg, AM ;
Kang, I ;
Johnson, S ;
Missalla, T ;
Chang, Z ;
Falcone, RW ;
Schoenlein, RW ;
Glover, TE ;
Padmore, HA .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT, 2001, 467 :986-989
[10]  
JOHNSON SL, 2002, THESIS U CALIFORNIA