Role of nitrogen-containing organic compound in plasma exhaust treatment

被引:7
作者
Nie, Yong [1 ]
Wang, Jingyi
Zhong, Kan
Wang, Liming
Guan, Zhicheng
机构
[1] Zhejiang Univ Technol, Coll Chem Engn & Mat Sci, Hangzhou 310014, Peoples R China
[2] Tsing Hua Univ, Grad Sch, Guangdong 518055, Peoples R China
基金
中国国家自然科学基金;
关键词
nitrogen-containing organic compounds; plasma-facilitated catalysis; NOx; N-2; selectivity;
D O I
10.1016/j.catcom.2007.07.019
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Role of nitrogen-containing organic compounds produced during the plasma process on the subsequent Of C2H4-SCR of NOx over Ag/gamma-Al2O3 catalyst at 523 K was studied in a two-stage plasma-facilitated catalysis system. Results showed that nitrogen-containing organic compounds (methyl nitrate, ethyl nitrate, nitro methyl) produced in the plasma reactor can improve the subsequent catalytic performance at lower temperature besides NO2 and aldehyde; more the amounts of nitrogen-containing organic compounds produced after plasma pretreatment, more the amounts of N-2 produced in the subsequent catalysis process, and N-2 selectivity leveled at about 82%. (c) 2007 Elsevier B.V. All rights reserved.
引用
收藏
页码:2153 / 2158
页数:6
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