New approach for determination of diffusion parameters of adatoms

被引:184
作者
Bott, M [1 ]
Hohage, M [1 ]
Morgenstern, M [1 ]
Michely, T [1 ]
Comsa, G [1 ]
机构
[1] FORSCHUNGSZENTRUM JULICH, FORSCHUNGSZENTRUM, INST GRENZFLACHENFORSCH & VAKUUMPHYS, D-52425 JULICH, GERMANY
关键词
D O I
10.1103/PhysRevLett.76.1304
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
A new approach for the determination of activation energy and attempt frequency for the diffusion of single adatoms on a surface is proposed and demonstrated for Pt adatom diffusion on Pt(lll). The method is based on a combination of low temperature scanning tunneling microscopy (STM) measurements and kinetic Monte Carlo simulations. The method involves only a minimum of assumptions and is independent of classical nucleation theory. This independence allows one to analyze the applicability of the latter. In addition, it is found that the measurement of the mean square displacement of individual adatoms is influenced by the STM tip.
引用
收藏
页码:1304 / 1307
页数:4
相关论文
共 26 条
[1]   DYNAMIC SCALING OF THE ISLAND-SIZE DISTRIBUTION AND PERCOLATION IN A MODEL OF SUBMONOLAYER MOLECULAR-BEAM EPITAXY [J].
AMAR, JG ;
FAMILY, F ;
LAM, PM .
PHYSICAL REVIEW B, 1994, 50 (12) :8781-8797
[2]   DYNAMICS OF IRREVERSIBLE ISLAND GROWTH DURING SUBMONOLAYER EPITAXY [J].
BALES, GS ;
CHRZAN, DC .
PHYSICAL REVIEW B, 1994, 50 (09) :6057-6067
[3]   SCALING ANALYSIS OF DIFFUSION-MEDIATED ISLAND GROWTH IN SURFACE-ADSORPTION PROCESSES [J].
BARTELT, MC ;
EVANS, JW .
PHYSICAL REVIEW B, 1992, 46 (19) :12675-12687
[4]   DIFFUSION OF SINGLE ADATOMS OF PLATINUM, IRIDIUM AND GOLD ON PLATINUM SURFACES [J].
BASSETT, DW ;
WEBBER, PR .
SURFACE SCIENCE, 1978, 70 (01) :520-531
[5]   DESIGN PRINCIPLES OF A VARIABLE-TEMPERATURE SCANNING TUNNELING MICROSCOPE [J].
BOTT, M ;
MICHELY, T ;
COMSA, G .
REVIEW OF SCIENTIFIC INSTRUMENTS, 1995, 66 (08) :4135-4139
[6]   MICROSCOPIC VIEW OF NUCLEATION ON SURFACES [J].
BRUNE, H ;
RODER, H ;
BORAGNO, C ;
KERN, K .
PHYSICAL REVIEW LETTERS, 1994, 73 (14) :1955-1958
[7]   SCANNING-TUNNELING-MICROSCOPE TIP-INDUCED MIGRATION OF VACANCIES ON GAP(110) [J].
EBERT, P ;
LAGALLY, MG ;
URBAN, K .
PHYSICAL REVIEW LETTERS, 1993, 70 (10) :1437-1440
[8]   ATOMIC VIEW OF SURFACE SELF-DIFFUSION - TUNGSTEN ON TUNGSTEN [J].
EHRLICH, G ;
HUDDA, FG .
JOURNAL OF CHEMICAL PHYSICS, 1966, 44 (03) :1039-&
[9]   ENERGETICS OF PT ADSORPTION ON PT(111) [J].
FEIBELMAN, PJ ;
NELSON, JS ;
KELLOGG, GL .
PHYSICAL REVIEW B, 1994, 49 (15) :10548-10556
[10]  
HOHAGE M, IN PRESS