Adsorption dynamics and effects of carbon to zeolite ratio of layered beds for multicomponent gas adsorption

被引:25
作者
Jang, Seong-Cheol [1 ,2 ]
Yang, Se-Il [1 ]
Oh, Seong-Geun [2 ]
Choi, Dae-Ki [1 ]
机构
[1] Korea Inst Sci & Technol, Fuel Cell Ctr, Seoul 136791, South Korea
[2] Hanyang Univ, Seoul 133791, South Korea
关键词
Adsorption Dynamic; Layered Bed; Carbon to Zeolite Ratio; Hydrogen; Dual-Site Langmuir; PRESSURE SWING ADSORPTION; OPTIMAL-DESIGN; SEPARATION; MIXTURES; PSA;
D O I
10.1007/s11814-010-0399-9
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
To optimize the performance of an adsorption bed, layered beds of activated carbon and zeolite 5A are used for multicomponent gas separation (H-2: 72.2%, CO2: 21.6%, CO: 2.03%, CH4: 4.17%). The adsorption dynamic characteristics were studied experimentally and theoretically using layered beds of activated carbon and zeolite 5A at 8 atm adsorption pressure and 16.67 L/min feed rate. Non-isothermal and non-adiabatic models, based on a linear driving force model and Dual-Site Langmuir adsorption isotherm model, were used. As the carbon ratio increased, the average velocity of CH4 wavefront became slow, and wavefronts of CO and CO2 propagated quickly on average.
引用
收藏
页码:583 / 590
页数:8
相关论文
共 23 条
[21]   Separation of hydrogen mixtures by a two-bed pressure swing adsorption process using zeolite 5A [J].
Yang, JY ;
Lee, CH ;
Chang, JW .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 1997, 36 (07) :2789-2798
[22]   Adsorption dynamics of a layered bed PSA for H2 recovery from coke oven gas [J].
Yang, JY ;
Lee, CH .
AICHE JOURNAL, 1998, 44 (06) :1325-1334
[23]  
Yang R.T., 1987, GAS SEPARATION ADSOR