Excitation and fragmentation mechanisms in ion-fullerene collisions

被引:85
作者
Kunert, T [1 ]
Schmidt, R [1 ]
机构
[1] Tech Univ Dresden, Inst Theoret Phys, D-01062 Dresden, Germany
关键词
D O I
10.1103/PhysRevLett.86.5258
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Electronic and vibronic excitations as well as fragmentation mechanisms in high energy ion (H+, C+, Ar+) fullerene collisions are investigated within a fully microscopic approach, called nonadiabatic quantum molecular dynamics. The total kinetic energy loss of the projectile depends dramatically on ion mass, but, surprisingly, does not depend on the impact velocity for all ions in a certain range. This is in striking contrast to the predictions of the "stopping power" concept of solids, but explains apparently contradicting experimental observations. Signatures for nonstatistical fragmentation mechanisms are predicted.
引用
收藏
页码:5258 / 5261
页数:4
相关论文
共 24 条
[1]   Internal energy dependence of the fragmentation patterns of C-60 and C-60(+) [J].
Campbell, EEB ;
Raz, T ;
Levine, RD .
CHEMICAL PHYSICS LETTERS, 1996, 253 (3-4) :261-267
[2]   Fullerene reactions [J].
Campbell, EEB ;
Rohmund, F .
REPORTS ON PROGRESS IN PHYSICS, 2000, 63 (07) :1061-1109
[3]   Electronic response of C60 in slow collisions with highly charged ions -: art. no. 022712 [J].
Cederquist, H ;
Fardi, A ;
Haghighat, K ;
Langereis, A ;
Schmidt, HT ;
Schwartz, H ;
Levin, JC ;
Sellin, IA ;
Lebius, H ;
Huber, B ;
Larsson, MO ;
Hvelplund, P .
PHYSICAL REVIEW A, 2000, 61 (02) :17
[4]   COLLISIONAL DYNAMICS OF C-60 WITH NOBLE-GAS-ATOMS STUDIED BY MOLECULAR-DYNAMICS WITH EMPIRICAL 2-BODY AND 3-BODY FORCES [J].
EHLICH, R ;
CAMPBELL, EEB ;
KNOSPE, O ;
SCHMIDT, R .
ZEITSCHRIFT FUR PHYSIK D-ATOMS MOLECULES AND CLUSTERS, 1993, 28 (02) :153-161
[5]   Molecular dynamics studies of inelastic scattering and fragmentation in collisions of C60 with rare-gas atoms [J].
Ehlich, R ;
Knospe, O ;
Schmidt, R .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 1997, 30 (23) :5429-5449
[6]   Fragmentation, charge transfer and chemical reactions in C60+/C70+-SF6 collisions [J].
Ehlich, R ;
Sprang, H ;
Westerburg, M ;
Campbell, EEB .
JOURNAL OF CHEMICAL PHYSICS, 1998, 108 (22) :9390-9397
[7]   Detailed experimental and theoretical study of collision-induced dissociation of Na2+ ions on He and H2 targets at keV energies [J].
Fayeton, JA ;
Barat, M ;
Brenot, JC ;
Dunet, H ;
Picard, YJ ;
Saalmann, U ;
Schmidt, R .
PHYSICAL REVIEW A, 1998, 57 (02) :1058-1068
[8]   DYNAMIC FRAGMENTATION OF C-60 IONS [J].
HVELPLUND, P ;
ANDERSEN, LH ;
HAUGEN, HK ;
LINDHARD, J ;
LORENTS, DC ;
MALHOTRA, R ;
RUOFF, R .
PHYSICAL REVIEW LETTERS, 1992, 69 (13) :1915-1918
[9]   Charge transfer and fragmentation in cluster-atom collisions [J].
Knospe, O ;
Jellinek, J ;
Saalmann, U ;
Schmidt, R .
PHYSICAL REVIEW A, 2000, 61 (02) :11
[10]   Charge transfer in cluster-atom collisions [J].
Knospe, O ;
Jellinek, J ;
Saalmann, U ;
Schmidt, R .
EUROPEAN PHYSICAL JOURNAL D, 1999, 5 (01) :1-4