Excitation and fragmentation mechanisms in ion-fullerene collisions

被引:85
作者
Kunert, T [1 ]
Schmidt, R [1 ]
机构
[1] Tech Univ Dresden, Inst Theoret Phys, D-01062 Dresden, Germany
关键词
D O I
10.1103/PhysRevLett.86.5258
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Electronic and vibronic excitations as well as fragmentation mechanisms in high energy ion (H+, C+, Ar+) fullerene collisions are investigated within a fully microscopic approach, called nonadiabatic quantum molecular dynamics. The total kinetic energy loss of the projectile depends dramatically on ion mass, but, surprisingly, does not depend on the impact velocity for all ions in a certain range. This is in striking contrast to the predictions of the "stopping power" concept of solids, but explains apparently contradicting experimental observations. Signatures for nonstatistical fragmentation mechanisms are predicted.
引用
收藏
页码:5258 / 5261
页数:4
相关论文
共 24 条
[11]  
KNOSPE O, 1999, THEORY ATOMIC MOL CL
[12]  
Larsen MC, 1999, EUR PHYS J D, V5, P283, DOI 10.1007/s100530050257
[13]  
Lindhard J, 1968, KGL DANSKE VIDENSKAB, V36, P1
[14]   Excitation and fragmentation of C60r+ (r=3-9) in Xe30+-C60 collisions -: art. no. 022707 [J].
Martin, S ;
Chen, L ;
Denis, A ;
Bredy, R ;
Bernard, J ;
Désesquelles, J .
PHYSICAL REVIEW A, 2000, 62 (02)
[15]   Electronic excitation in H+-C60 collisions:: Evaporation and ionization -: art. no. 022705 [J].
Opitz, J ;
Lebius, H ;
Tomita, S ;
Huber, BA ;
Capelle, PM ;
Montesquieu, DB ;
Montesquieu, AB ;
Reinköster, A ;
Werner, U ;
Lutz, HO ;
Niehaus, A ;
Benndorf, M ;
Haghighat, K ;
Schmidt, HT ;
Cederquist, H .
PHYSICAL REVIEW A, 2000, 62 (02) :10
[16]   Ion-impact-induced C60 fragmentation [J].
Reinkoster, A ;
Werner, U ;
Lutz, HO .
EUROPHYSICS LETTERS, 1998, 43 (06) :653-658
[17]   Strong temperature dependence of laser-enhanced charge transfer in collisions of sodium clusters with sodium atoms [J].
Roller-Lutz, Z ;
Wang, Y ;
Lutz, HO ;
Saalmann, U ;
Schmidt, R .
PHYSICAL REVIEW A, 1999, 59 (04) :R2555-R2558
[18]   DENSITY-FUNCTIONAL THEORY FOR TIME-DEPENDENT SYSTEMS [J].
RUNGE, E ;
GROSS, EKU .
PHYSICAL REVIEW LETTERS, 1984, 52 (12) :997-1000
[19]   Excitation and relaxation in atom-cluster collisions [J].
Saalmann, U ;
Schmidt, R .
PHYSICAL REVIEW LETTERS, 1998, 80 (15) :3213-3216
[20]   Non-adiabatic quantum molecular dynamics: Basic formalism and case study [J].
Saalmann, U ;
Schmidt, R .
ZEITSCHRIFT FUR PHYSIK D-ATOMS MOLECULES AND CLUSTERS, 1996, 38 (02) :153-163