Air pollutant emissions from Chinese households: A major and underappreciated ambient pollution source

被引:412
作者
Liu, Jun [1 ]
Mauzerall, Denise L. [2 ,3 ]
Chen, Qi [1 ]
Zhang, Qiang [4 ]
Song, Yu [1 ]
Peng, Wei [2 ]
Klimont, Zbigniew [5 ]
Qiu, Xinghua [1 ]
Zhang, Shiqiu [1 ]
Hu, Min [1 ]
Lin, Weili [6 ]
Smith, Kirk R. [7 ]
Zhu, Tong [1 ,8 ]
机构
[1] Peking Univ, Coll Environm Sci & Engn, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100871, Peoples R China
[2] Princeton Univ, Woodrow Wilson Sch Publ & Int Affairs, Princeton, NJ 08544 USA
[3] Princeton Univ, Dept Civil & Environm Engn, Princeton, NJ 08544 USA
[4] Tsinghua Univ, Ctr Earth Syst Sci, Key Lab Earth Syst Modeling, Minist Educ, Beijing 100084, Peoples R China
[5] IIASA, Schlosspl 1, A-2361 Laxenburg, Austria
[6] Chinese Acad Meteorol Sci, Beijing 100081, Peoples R China
[7] Univ Calif Berkeley, Sch Publ Hlth, Berkeley, CA 94720 USA
[8] Peking Univ, Beijing Innovat Ctr Engn Sci & Adv Technol, Beijing 100871, Peoples R China
关键词
PM2.5; secondary aerosols; regional pollution transport; residential emissions; source contribution; COMPARATIVE RISK-ASSESSMENT; SULFUR-DIOXIDE; CARBONACEOUS PARTICLES; CHEMICAL-COMPOSITIONS; SOURCE APPORTIONMENT; PARTICULATE MATTER; NORTH CHINA; PM2.5; MODEL; IMPACTS;
D O I
10.1073/pnas.1604537113
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
As part of the 12th Five-Year Plan, the Chinese government has developed air pollution prevention and control plans for key regions with a focus on the power, transport, and industrial sectors. Here, we investigate the contribution of residential emissions to regional air pollution in highly polluted eastern China during the heating season, and find that dramatic improvements in air quality would also result from reduction in residential emissions. We use the Weather Research and Forecasting model coupled with Chemistry to evaluate potential residential emission controls in Beijing and in the Beijing, Tianjin, and Hebei (BTH) region. In January and February 2010, relative to the base case, eliminating residential emissions in Beijing reduced daily average surface PM2.5 (particulate mater with aerodynamic diameter equal or smaller than 2.5 micrometer) concentrations by 14 +/- 7 mu g.m(-3) (22 +/- 6% of a baseline concentration of 67 +/- 41 mu g.m(-3); mean +/- SD). Eliminating residential emissions in the BTH region reduced concentrations by 28 +/- 19 mu g.m(-3) (40 +/- 9% of 67 +/- 41 mu g.m(-3)), 44 +/- 27 mu g.m(-3) (43 +/- 10% of 99 +/- 54 mu g.m(-3)), and 25 +/- 14 mu g.m(-3) (35 +/- 8% of 70 +/- 35 mu g.m(-3)) in Beijing, Tianjin, and Hebei provinces, respectively. Annually, elimination of residential sources in the BTH region reduced emissions of primary PM2.5 by 32%, compared with 5%, 6%, and 58% achieved by eliminating emissions from the transportation, power, and industry sectors, respectively. We also find air quality in Beijing would benefit substantially from reductions in residential emissions from regional controls in Tianjin and Hebei, indicating the value of policies at the regional level.
引用
收藏
页码:7756 / 7761
页数:6
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