Global and regional evolution of short-lived radiatively-active gases and aerosols in the Representative Concentration Pathways

被引:355
作者
Lamarque, Jean-Francois [1 ]
Kyle, G. Page [2 ]
Meinshausen, Malte [3 ]
Riahi, Keywan [4 ]
Smith, Steven J. [2 ]
van Vuuren, Detlef P. [5 ,6 ]
Conley, Andrew J. [1 ]
Vitt, Francis [1 ]
机构
[1] Natl Ctr Atmospher Res, Boulder, CO 80307 USA
[2] Pacific NW Natl Lab, Joint Global Change Res Inst, College Pk, MD USA
[3] Potsdam Inst Climate Impact Res, Potsdam, Germany
[4] Int Inst Appl Syst Anal, A-2361 Laxenburg, Austria
[5] Netherlands Environm Assessment Agcy, Utrecht, Netherlands
[6] Univ Utrecht, Utrecht, Netherlands
基金
美国国家科学基金会;
关键词
GENERAL-CIRCULATION MODEL; NITROGEN DEPOSITION; MULTIMODEL ASSESSMENT; OZONE POLLUTION; CLIMATE-CHANGE; UNITED-STATES; BLACK CARBON; PREINDUSTRIAL; EMISSIONS; CHEMISTRY;
D O I
10.1007/s10584-011-0155-0
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
In this paper, we discuss the results of 2000-2100 simulations following the emissions associated with the Representative Concentration Pathways (RCPs) with a chemistry-climate model, focusing on the changes in 1) atmospheric composition (troposphere and stratosphere) and 2) associated environmental parameters (such as nitrogen deposition). In particular, we find that tropospheric ozone is projected to decrease (RCP2.6, RCP4.5 and RCP6) or increase (RCP8.5) between 2000 and 2100, with variations in methane a strong contributor to this spread. The associated tropospheric ozone global radiative forcing is shown to be in agreement with the estimate used in the RCPs, except for RCP8.5. Surface ozone in 2100 is projected to change little compared from its 2000 distribution, a much-reduced impact from previous projections based on the A2 high-emission scenario. In addition, globally-averaged stratospheric ozone is projected to recover at or beyond pre-1980 levels. Anthropogenic aerosols are projected to strongly decrease in the 21st century, a reflection of their projected decrease in emissions. Consequently, sulfate deposition is projected to strongly decrease. However, nitrogen deposition is projected to increase over certain regions because of the projected increase in NH3 emissions.
引用
收藏
页码:191 / 212
页数:22
相关论文
共 75 条
[1]   General circulation model assessment of direct radiative forcing by the sulfate-nitrate-ammonium-water inorganic aerosol system [J].
Adams, PJ ;
Seinfeld, JH ;
Koch, D ;
Mickley, L ;
Jacob, D .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2001, 106 (D1) :1097-1111
[2]   Intercontinental Impacts of Ozone Pollution on Human Mortality [J].
Anenberg, Susan Casper ;
West, J. Jason ;
Fiore, Arlene M. ;
Jaffe, Daniel A. ;
Prather, Michael J. ;
Bergmann, Daniel ;
Cuvelier, Kees ;
Dentener, Frank J. ;
Duncan, Bryan N. ;
Gauss, Michael ;
Hess, Peter ;
Jonson, Jan Eiof ;
Lupu, Alexandru ;
MacKenzie, Ian A. ;
Marmer, Elina ;
Park, Rokjin J. ;
Sanderson, Michael G. ;
Schultz, Martin ;
Shindell, Drew T. ;
Szopa, Sophie ;
Garcia Vivanco, Marta ;
Wild, Oliver ;
Zang, Guang .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2009, 43 (17) :6482-6487
[3]  
[Anonymous], ATMOS CHEM PHYS DISC
[4]  
[Anonymous], CLIMATE CHANGE 2007
[5]  
[Anonymous], 2009, CMIP Report
[6]  
[Anonymous], PUBLICATION JET PROP
[7]   Chemistry-climate model simulations of spring Antarctic ozone [J].
Austin, John ;
Struthers, H. ;
Scinocca, J. ;
Plummer, D. A. ;
Akiyoshi, H. ;
Baumgaertner, A. J. G. ;
Bekki, S. ;
Bodeker, G. E. ;
Braesicke, P. ;
Bruehl, C. ;
Butchart, N. ;
Chipperfield, M. P. ;
Cugnet, D. ;
Dameris, M. ;
Dhomse, S. ;
Frith, S. ;
Garny, H. ;
Gettelman, A. ;
Hardiman, S. C. ;
Joeckel, P. ;
Kinnison, D. ;
Kubin, A. ;
Lamarque, J. F. ;
Langematz, U. ;
Mancini, E. ;
Marchand, M. ;
Michou, M. ;
Morgenstern, O. ;
Nakamura, T. ;
Nielsen, J. E. ;
Pitari, G. ;
Pyle, J. ;
Rozanov, E. ;
Shepherd, T. G. ;
Shibata, K. ;
Smale, D. ;
Teyssedre, H. ;
Yamashita, Y. .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2010, 115
[8]   Sulfur chemistry in the National Center for Atmospheric Research Community Climate Model: Description, evaluation, features, and sensitivity to aqueous chemistry [J].
Barth, MC ;
Rasch, PJ ;
Kiehl, JT ;
Benkovitz, CM ;
Schwartz, SE .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2000, 105 (D1) :1387-1415
[9]   The effects of air-borne nitrogen pollutants on species diversity in natural and semi-natural European vegetation [J].
Bobbink, R ;
Hornung, M ;
Roelofs, JGM .
JOURNAL OF ECOLOGY, 1998, 86 (05) :717-738
[10]   A global analysis of acidification and eutrophication of terrestrial ecosystems [J].
Bouwman, AF ;
Van Vuuren, DP ;
Derwent, RG ;
Posch, M .
WATER AIR AND SOIL POLLUTION, 2002, 141 (1-4) :349-382