Quantum mode-coupling theory: Formulation and applications to normal and supercooled quantum liquids

被引:34
作者
Rabani, E [1 ]
Reichman, DR
机构
[1] Tel Aviv Univ, Sackler Fac Exact Sci, Sch Chem, IL-69978 Tel Aviv, Israel
[2] Harvard Univ, Dept Chem & Biol Chem, Cambridge, MA 02138 USA
关键词
quantum dynamics; normal and supercooled quantum liquids; path integral Monte Carlo;
D O I
10.1146/annurev.physchem.56.092503.141138
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We review our recent efforts to formulate and study a mode-coupling approach to real-time dynamic fluctuations in quantum liquids. Comparison is made between the theory and recent neutron scattering experiments performed on liquid ortho-deuterium and para-hydrogen. We discuss extensions of the theory to supercooled and glassy states where quantum fluctuations compete with thermal fluctuations. Experimental scenarios for quantum glassy liquids are briefly discussed.
引用
收藏
页码:157 / 185
页数:29
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