Quantum mode-coupling theory: Formulation and applications to normal and supercooled quantum liquids

被引：34

作者：

Rabani, E ^{[1
]}

Reichman, DR

机构：

[1] Tel Aviv Univ, Sackler Fac Exact Sci, Sch Chem, IL-69978 Tel Aviv, Israel

[2] Harvard Univ, Dept Chem & Biol Chem, Cambridge, MA 02138 USA

来源：

ANNUAL REVIEW OF PHYSICAL CHEMISTRY | 2005年 / 56卷

关键词：

quantum dynamics; normal and supercooled quantum liquids; path integral Monte Carlo;

D O I：

10.1146/annurev.physchem.56.092503.141138

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

We review our recent efforts to formulate and study a mode-coupling approach to real-time dynamic fluctuations in quantum liquids. Comparison is made between the theory and recent neutron scattering experiments performed on liquid ortho-deuterium and para-hydrogen. We discuss extensions of the theory to supercooled and glassy states where quantum fluctuations compete with thermal fluctuations. Experimental scenarios for quantum glassy liquids are briefly discussed.

引用

页码：157 / 185

页数：29

共 118 条

[61] Aging dynamics of quantum spin glasses of rotors [J].

Kennett, MP ;

Chamon, C ;

Ye, JW .

PHYSICAL REVIEW B, 2001, 64 (22)

[62] Path integral centroid molecular dynamics study of the dynamic structure factors of liquid para-hydrogen [J].

Kinugawa, K .

CHEMICAL PHYSICS LETTERS, 1998, 292 (4-6) :454-460

[63] Quantitative tests of mode-coupling theory for fragile and strong glass formers [J].

Kob, W ;

Nauroth, M ;

Sciortino, F .

JOURNAL OF NON-CRYSTALLINE SOLIDS, 2002, 307 :181-187

[64] Computer simulations of supercooled liquids and glasses [J].

Kob, W .

JOURNAL OF PHYSICS-CONDENSED MATTER, 1999, 11 (10) :R85-R115

[65] TESTING MODE-COUPLING THEORY FOR A SUPERCOOLED BINARY LENNARD-JONES MIXTURE - THE VAN HOVE CORRELATION-FUNCTION [J].

KOB, W ;

ANDERSEN, HC .

PHYSICAL REVIEW E, 1995, 51 (05) :4626-4641

[66] TESTING MODE-COUPLING THEORY FOR A SUPERCOOLED BINARY LENNARD-JONES MIXTURE .2. INTERMEDIATE SCATTERING FUNCTION AND DYNAMIC SUSCEPTIBILITY [J].

KOB, W ;

ANDERSEN, HC .

PHYSICAL REVIEW E, 1995, 52 (04) :4134-4153

[67] On the Bayesian approach to calculating time correlation functions in quantum systems; reaction dynamics and spectroscopy [J].

Krilov, G ;

Sim, E ;

Berne, BJ .

CHEMICAL PHYSICS, 2001, 268 (1-3) :21-34

[68] ADIABATIC APPROXIMATION AND NONADIABATIC EFFECTS FOR OPEN-SHELL ATOMS IN AN INERT SOLVENT - F-ATOMS IN SOLID KR [J].

KRYLOV, AI ;

GERBER, RB ;

APKARIAN, VA .

CHEMICAL PHYSICS, 1994, 189 (02) :261-272

[69] Reexamination of the mode-coupling scheme for the glass transition [J].

Liu, CZW ;

Oppenheim, I .

PHYSICA A, 1997, 235 (3-4) :369-387

[70] Forward-backward quantum dynamics for time correlation functions [J].

Makri, N .

JOURNAL OF PHYSICAL CHEMISTRY A, 2004, 108 (05) :806-812

← 2 3 4 5 6 7 8 9 10 11 →