An Amine-Functionalized Titanium Metal-Organic Framework Photocatalyst with Visible-Light-Induced Activity for CO2 Reduction

被引：1556

作者：

Fu, Yanghe ^{[1
]}

Sun, Dengrong ^{[1
]}

Chen, Yongjuan ^{[1
]}

Huang, Renkun ^{[1
]}

Ding, Zhengxin ^{[1
]}

Fu, Xianzhi ^{[1
]}

Li, Zhaohui ^{[1
]}

机构：

[1] Fuzhou Univ, State Key Lab Breeding Base, Res Inst Photocatalysis, Fujian Prov Key Lab Photocatalysis, Fuzhou 350002, Peoples R China

来源：

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION | 2012年 / 51卷 / 14期

基金：

中国国家自然科学基金;

关键词：

carbon dioxide; metal-organic frameworks; photocatalysis; reduction; CARBON-DIOXIDE; ROOM-TEMPERATURE; WATER; MOFS; BEHAVIOR; ACID;

D O I：

10.1002/anie.201108357

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Let your light shine: The photocatalytic reduction of carbon dioxide to the formate anion under visible light irradiation is for the first time realized over a photoactive Ti-containing metal-organic framework, NH 2-MIL- 125(Ti), which is fabricated by a facile substitution of ligands in the UV-responsive MIL-125(Ti) material (see scheme; TEOA=triethanolamine). Copyright © 2012 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

引用

页码：3364 / 3367

页数：4

共 46 条

[41]

Yamashita H., 2002, CO2 CONVERS UTIL, V22, P330

[42]

Yan S.C., 2010, ANGEW CHEM, V122, P6544, DOI DOI 10.1002/ANGE.201003270

[43] A Room-Temperature Reactive-Template Route to Mesoporous ZnGa2O4 with Improved Photocatalytic Activity in Reduction of CO2 [J].

Yan, Shi Cheng ;

Ouyang, Shu Xin ;

Gao, Jun ;

Yang, Ming ;

Feng, Jian Yong ;

Fan, Xiao Xing ;

Wan, Li Juan ;

Li, Zhao Sheng ;

Ye, Jin Hua ;

Zhou, Yong ;

Zou, Zhi Gang .

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2010, 49 (36) :6400-6404

[44]

Yuan B. Z., 2010, ANGEW CHEM, V122, P4148

[45] A Highly Active Heterogeneous Palladium Catalyst for the Suzuki-Miyaura and Ullmann Coupling Reactions of Aryl Chlorides in Aqueous Media [J].

Yuan, Bizhen ;

Pan, Yingyi ;

Li, Yingwei ;

Yin, Biaolin ;

Jiang, Huanfeng .

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2010, 49 (24) :4054-4058

[46] Effect of NH2 and CF3 functionalization on the hydrogen sorption properties of MOFs [J].

Zlotea, Claudia ;

Phanon, Delphine ;

Mazaj, Matjaz ;

Heurtaux, Daniela ;

Guillerm, Vincent ;

Serre, Christian ;

Horcajada, Patricia ;

Devic, Thomas ;

Magnier, Emmanuel ;

Cuevas, Fermin ;

Ferey, Gerard ;

Llewellyn, Philip L. ;

Latroche, Michel .

DALTON TRANSACTIONS, 2011, 40 (18) :4879-4881

← 1 2 3 4 5 →