Generation of tunable octave-spanning mid-infrared pulses by filamentation in gas media

被引:33
作者
Cheng, Mark [1 ]
Reynolds, Anthony [1 ]
Widgren, Heather [1 ]
Khalil, Munira [1 ]
机构
[1] Univ Washington, Dept Chem, Seattle, WA 98195 USA
基金
美国国家科学基金会;
关键词
AIR;
D O I
10.1364/OL.37.001787
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
The continued development of femtosecond mid-infrared (IR) sources with ultrabroad spectral width is critical for probing and controlling complex molecular structural dynamics on an ultrafast timescale. We report on a sub-20 fs, coherent mid-IR source with an octave-spanning spectral bandwidth (>2000 cm(-1)) tunable from 2-8 micrometers (37.5-150 THz), with energy >0.4 mu J/pulse at 1 kHz. The mid-IR pulses are generated by four-wave mixing during the filamentation of intense 800 nm and 400 nm pulses in various gas media. Spectral tunability is achieved by the choice of gas, pressure and input 800 nm pulse energy. (C) 2012 Optical Society of America
引用
收藏
页码:1787 / 1789
页数:3
相关论文
共 17 条
[1]   Ultrabroadband detection of a mid-IR continuum by chirped-pulse upconversion [J].
Baiz, Carlos R. ;
Kubarych, Kevin J. .
OPTICS LETTERS, 2011, 36 (02) :187-189
[2]   Advances in intense femtosecond laser filamentation in air [J].
Chin, S. L. ;
Wang, T. -J. ;
Marceau, C. ;
Wu, J. ;
Liu, J. S. ;
Kosareva, O. ;
Panov, N. ;
Chen, Y. P. ;
Daigle, J. -F. ;
Yuan, S. ;
Azarm, A. ;
Liu, W. W. ;
Seideman, T. ;
Zeng, H. P. ;
Richardson, M. ;
Li, R. ;
Xu, Z. Z. .
LASER PHYSICS, 2012, 22 (01) :1-53
[3]   Intense terahertz pulses by four-wave rectification in air [J].
Cook, DJ ;
Hochstrasser, RM .
OPTICS LETTERS, 2000, 25 (16) :1210-1212
[4]   Dispersion compensation with optical materials for compression of intense sub-100-fs mid-infrared pulses [J].
Demirdöven, N ;
Khalil, M ;
Golonzka, O ;
Tokmakoff, A .
OPTICS LETTERS, 2002, 27 (06) :433-435
[5]   Generation of sub-two-cycle mid-infrared pulses by four-wave mixing through filamentation in air [J].
Fuji, Takao ;
Suzuki, Toshinori .
OPTICS LETTERS, 2007, 32 (22) :3330-3332
[6]   Generation, shaping, and characterization of intense femtosecond pulses tunable from 3 to 20 μm [J].
Kaindl, RA ;
Wurm, M ;
Reimann, K ;
Hamm, P ;
Weiner, AM ;
Woerner, M .
JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS, 2000, 17 (12) :2086-2094
[7]   Coherent control of terahertz supercontinuum generation in ultrafast laser-gas interactions [J].
Kim, K. Y. ;
Taylor, A. J. ;
Glownia, J. H. ;
Rodriguez, G. .
NATURE PHOTONICS, 2008, 2 (10) :605-609
[8]   Infrared generation by filamentation in air of a spectrally shaped laser beam [J].
Lassonde, P. ;
Theberge, F. ;
Payeur, S. ;
Chateauneuf, M. ;
Dubois, J. ;
Kieffer, J. -C. .
OPTICS EXPRESS, 2011, 19 (15) :14093-14098
[9]  
Linden S, 1998, PHYS STATUS SOLIDI B, V206, P119, DOI 10.1002/(SICI)1521-3951(199803)206:1<119::AID-PSSB119>3.0.CO
[10]  
2-X