Carbon dioxide sequestration in deep-sea basalt

被引:240
作者
Goldberg, David S. [1 ]
Takahashi, Taro [1 ]
Slagle, Angela L. [1 ]
机构
[1] Columbia Univ, Lamont Doherty Geol Observ, Palisades, NY 10964 USA
关键词
climate change; ocean crust; climate mitigation; fossil fuel emissions; energy;
D O I
10.1073/pnas.0804397105
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Developing a method for secure sequestration of anthropogenic carbon dioxide in geological formations is one of our most pressing global scientific problems. Injection into deep-sea basalt formations provides unique and significant advantages over other potential geological storage options, including (i) vast reservoir capacities sufficient to accommodate centuries-long U.S. production of fossil fuel CO2 at locations within pipeline distances to populated areas and CO2 sources along the U.S. west coast; (ii) sufficiently closed water-rock circulation pathways for the chemical reaction of CO2 with basalt to produce stable and nontoxic (Ca2+, Mg2+, Fe2+)CO3 infilling minerals, and (iii) significant risk reduction for post-injection leakage by geological, gravitational, and hydrate-trapping mechanisms. CO2 sequestration in established sediment-covered basalt aquifers on the Juan de Fuca plate offer promising locations to securely accommodate more than a century of future U.S. emissions, warranting energized scientific research, technological assessment, and economic evaluation to establish a viable pilot injection program in the future.
引用
收藏
页码:9920 / 9925
页数:6
相关论文
共 46 条
[11]   Borehole-to-borehole hydrologic response across 2.4 km in the upper oceanic crust: Implications for crustal-scale properties [J].
Fisher, A. T. ;
Davis, E. E. ;
Becker, K. .
JOURNAL OF GEOPHYSICAL RESEARCH-SOLID EARTH, 2008, 113 (B7)
[12]   Hydrothermal recharge and discharge across 50 km guided by seamounts on a young ridge flank [J].
Fisher, AT ;
Davis, EE ;
Hutnak, M ;
Spiess, V ;
Zühlsdorff, L ;
Cherkaoui, A ;
Christiansen, L ;
Edwards, K ;
Macdonald, R ;
Villinger, H ;
Mottl, MJ ;
Wheat, CG ;
Becker, K .
NATURE, 2003, 421 (6923) :618-621
[13]   The permeability of young oceanic crust east of Juan de Fuca Ridge determined using borehole thermal measurements [J].
Fisher, AT ;
Becker, K ;
Davis, EE .
GEOPHYSICAL RESEARCH LETTERS, 1997, 24 (11) :1311-1314
[14]   Permeability within basaltic oceanic crust [J].
Fisher, AT .
REVIEWS OF GEOPHYSICS, 1998, 36 (02) :143-182
[15]  
FISHER AT, 2005, SCI DRILLING, DOI [DOI 10.2204/IODP.SD.1.01, 10.2204/iodp.sd.1.01]
[16]   The role of downhole measurements in marine geology and geophysics [J].
Goldberg, D .
REVIEWS OF GEOPHYSICS, 1997, 35 (03) :315-342
[17]  
Goldberg D., 1999, INT J SOC MAT ENG, V7, P11
[18]  
Gunter W. D., 2004, GEOLOGICAL SOC SPECI, V233, P129, DOI [DOI 10.1144/GSL.SP.2004.233.01.09, 10.1144/GSL.SP.2004.233.01.09, https://doi.org/10.1144/GSL.SP.2004.233.01.09]
[19]   AQUIFER DISPOSAL OF CO2-RICH GASES - REACTION DESIGN FOR ADDED CAPACITY [J].
GUNTER, WD ;
PERKINS, EH .
ENERGY CONVERSION AND MANAGEMENT, 1993, 34 (9-11) :941-948
[20]   No exit: thinking about leakage from geologic carbon storage sites [J].
Hawkins, DG .
ENERGY, 2004, 29 (9-10) :1571-1578