Electrowetting in carbon nanotubes

被引:105
作者
Chen, JY [1 ]
Kutana, A [1 ]
Collier, CP [1 ]
Giapis, KP [1 ]
机构
[1] CALTECH, Div Chem & Chem Engn, Pasadena, CA 91125 USA
关键词
D O I
10.1126/science.1120385
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
We demonstrate reversible wetting and fitting of open single-watt carbon nanotubes with mercury by means of electrocapillary pressure originating from the application of a potential across an individual nanotube in contact with a mercury drop. Wetting improves the conductance in both metallic and semiconducting nanotube probes by decreasing contact resistance and forming a mercury nanowire inside the nanotube. Molecular dynamics simulations corroborate the electrocapillary-driven filling process and provide estimates for the imbibition speed and electrocapillary pressure.
引用
收藏
页码:1480 / 1483
页数:4
相关论文
共 28 条
[1]  
ADAM NK, 1968, PHYS CHEM SURFACES, P20601
[2]   CAPILLARITY-INDUCED FILLING OF CARBON NANOTUBES [J].
AJAYAN, PM ;
IIJIMA, S .
NATURE, 1993, 361 (6410) :333-334
[3]   Nanometre-size tubes of carbon [J].
Ajayan, PM ;
Ebbesen, TW .
REPORTS ON PROGRESS IN PHYSICS, 1997, 60 (10) :1025-1062
[4]   Measurement of contact angle in systems involving liquid metals [J].
Awasthi, A ;
Bhatt, YJ ;
Garg, SP .
MEASUREMENT SCIENCE AND TECHNOLOGY, 1996, 7 (05) :753-757
[5]  
Dujardin E, 1998, ADV MATER, V10, P1472, DOI 10.1002/(SICI)1521-4095(199812)10:17<1472::AID-ADMA1472>3.0.CO
[6]  
2-R
[7]   CAPILLARITY AND WETTING OF CARBON NANOTUBES [J].
DUJARDIN, E ;
EBBESEN, TW ;
HIURA, H ;
TANIGAKI, K .
SCIENCE, 1994, 265 (5180) :1850-1852
[8]   Wetting, filling and decorating carbon nanotubes [J].
Ebbesen, TW .
JOURNAL OF PHYSICS AND CHEMISTRY OF SOLIDS, 1996, 57 (6-8) :951-955
[9]   Absorption of mercury in gold films and its further desorption: Quantitative morphological study of the surface patterns [J].
Fialkowski, M ;
Grzeszczak, P ;
Nowakowski, R ;
Holyst, R .
JOURNAL OF PHYSICAL CHEMISTRY B, 2004, 108 (16) :5026-5030
[10]   Carbon nanotube quantum resistors [J].
Frank, S ;
Poncharal, P ;
Wang, ZL ;
de Heer, WA .
SCIENCE, 1998, 280 (5370) :1744-1746