Probing glasslike excitations in single-crystalline Sr8Ga16Ge30 by specific heat and thermal conductivity

被引:53
作者
Umeo, K [1 ]
Avila, MA
Sakata, T
Suekuni, K
Takabatake, T
机构
[1] Hiroshima Univ, ADSM, Dept Quantum Matter, Higashihiroshima, Hiroshima 7398530, Japan
[2] Hiroshima Univ, NBARD, Ctr Mat Sci, Higashihiroshima, Hiroshima 7398530, Japan
关键词
Sr8Ga16Ge30; clathrate; specific heat; thermal conductivity; soft-potential model;
D O I
10.1143/JPSJ.74.2145
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We report the thermal conductivity K and specific heat C measurements down to 0.3 K on single-crystalline samples of n-type Sr8Ga16Ge30 and p-type Ba8Ga16Ge30 clathrates. The overall temperature dependence of K(T) of both samples with a plateau at about 20 K and a quadratic T dependence below I K is well described by the soft-potential model. Using the soft-potential parameter of 4.4 K derived from the analysis Of K(T) for Sr8Ga16Ge30, the broad maximum of C/T-3 centered at 7 K is also well reproduced. The density of states of quasilocalized vibrational modes for Sr atoms in Sr8Ga16Ge30 has a maximum at 0.7 THz, in agreement with the low-energy peak in a previous Raman scattering study.
引用
收藏
页码:2145 / 2148
页数:4
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