Room-temperature ordered photon emission from multiexciton states in single CdSe core-shell nanocrystals

被引:154
作者
Fisher, B
Caruge, JM
Zehnder, D
Bawendi, M
机构
[1] MIT, Dept Chem, Cambridge, MA 02139 USA
[2] Quantum Dot Corp, Hayward, CA 94545 USA
关键词
D O I
10.1103/PhysRevLett.94.087403
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We report room-temperature ordered multiphoton emission from multiexciton states of single CdSe(CdZnS) core(-shell) colloidal nanocrystals (NCs) that are synthesized by wet chemical methods. Spectrally and temporally resolved measurements of biexciton and triexciton emission from single NCs are also presented. A simple four level system models the results accurately and provides estimates for biexciton and triexciton radiative lifetimes and quantum yields.
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页数:4
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