Voltage control of the spin dynamics of an exciton in a semiconductor quantum dot

被引:141
作者
Smith, JM [1 ]
Dalgarno, PA
Warburton, RJ
Govorov, AO
Karrai, K
Gerardot, BD
Petroff, PM
机构
[1] Heriot Watt Univ, Sch Engn & Phys Sci, Edinburgh EH14 4AS, Midlothian, Scotland
[2] Ohio Univ, Dept Phys & Astron, Athens, OH 45701 USA
[3] Univ Munich, Ctr NanoSci, D-80539 Munich, Germany
[4] Univ Munich, Dept Phys, D-80539 Munich, Germany
[5] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA
基金
英国工程与自然科学研究理事会;
关键词
D O I
10.1103/PhysRevLett.94.197402
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We report the observation of a spin-flip process in a quantum dot whereby a dark exciton with total angular momentum L=2 becomes a bright exciton with L=1. The spin-flip process is revealed in the decay dynamics following nongeminate excitation. We are able to control the spin-flip rate by more than an order of magnitude simply with a dc voltage. The spin-flip mechanism involves a spin exchange with the Fermi sea in the back contact of our device and corresponds to the high temperature Kondo regime. We use the Anderson Hamiltonian to calculate a spin-flip rate, and we find excellent agreement with the experimental results.
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页数:4
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