Specific chimney emissions and biofuel characteristics of softwood pellets for residential heating in Sweden

被引:44
作者
Olsson, M [1 ]
Kjällstrand, J [1 ]
Petersson, G [1 ]
机构
[1] Chalmers Univ Technol, Dept Chem Environm Sci, SE-41296 Gothenburg, Sweden
关键词
wood pellets; stoves; burners; benzene; PAH; phenols; biomass waste;
D O I
10.1016/S0961-9534(02)00083-1
中图分类号
S2 [农业工程];
学科分类号
0828 ;
摘要
Softwood pellets are mainly produced from sawdust and to some extent from wood shavings. The moisture content is typically less than half of that in firewood. The present annual residential use in Sweden for pellet burners in boilers and for pellet stoves amounts to more than 100 000 tonnes and is increasing rapidly. The total annual production capacity at the more than 20 units exceeds one million tonnes, and permits continued rapid replacement of firewood and petroleum oil for residential heating. With the purpose of characterising emissions to air, chimney smoke was sampled, and specific compounds were assessed by gas chromatography and mass spectrometry. Benzene was the predominant aromatic compound in emissions from pellet burners. The smoke from stoves contained methoxyphenols with antioxidant properties and lower proportions of aromatic hydrocarbons. Observed differences in emissions from specific burning appliances are of interest with regard to both health hazards and regulation of emissions. Consideration of ecological aspects and pollution hazards indicates that wood pellets should be used primarily for residential heating, whereas controlled large-scale combustion is preferable for most other types of biomass waste. (C) 2002 Elsevier Science Ltd. All rights reserved.
引用
收藏
页码:51 / 57
页数:7
相关论文
共 17 条
[1]   Formation of the main degradation compound groups from wood and its components during pyrolysis [J].
Alen, R ;
Kuoppala, E ;
Oesch, P .
JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS, 1996, 36 (02) :137-148
[2]   VOLATILE HYDROCARBONS FROM DOMESTIC WOOD BURNING [J].
BARREFORS, G ;
PETERSSON, G .
CHEMOSPHERE, 1995, 30 (08) :1551-1556
[3]   ASSESSMENT OF AMBIENT VOLATILE HYDROCARBONS FROM TOBACCO-SMOKE AND FROM VEHICLE EMISSIONS [J].
BARREFORS, G ;
PETERSSON, G .
JOURNAL OF CHROMATOGRAPHY, 1993, 643 (1-2) :71-76
[4]   COLLECTION AND QUANTITATION OF METHOXYLATED PHENOL TRACERS FOR ATMOSPHERIC-POLLUTION FROM RESIDENTIAL WOOD STOVES [J].
HAWTHORNE, SB ;
KRIEGER, MS ;
MILLER, DJ ;
MATHIASON, MB .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1989, 23 (04) :470-475
[5]   Abatement of emissions in small-scale combustors through utilisation of blended pellet fuels [J].
Heschel, W ;
Rweyemamu, L ;
Scheibner, T ;
Meyer, B .
FUEL PROCESSING TECHNOLOGY, 1999, 61 (03) :223-242
[6]  
Hillring B, 1998, FOREST PROD J, V48, P67
[7]   Methoxyphenols from burning of Scandinavian forest plant materials [J].
Kjällstrand, J ;
Ramnäs, O ;
Petersson, G .
CHEMOSPHERE, 2000, 41 (05) :735-741
[8]   Phenolic antioxidants in wood smoke [J].
Kjällstrand, J ;
Petersson, G .
SCIENCE OF THE TOTAL ENVIRONMENT, 2001, 277 (1-3) :69-75
[9]   Phenols and aromatic hydrocarbons in chimney emissions from traditional and modern residential wood burning [J].
Kjällstrand, J ;
Petersson, G .
ENVIRONMENTAL TECHNOLOGY, 2001, 22 (04) :391-395
[10]   PCDD/F- and PAH-emission from house heating systems [J].
Launhardt, T ;
Strehler, A ;
Dumler-Gradl, R ;
Thoma, H ;
Vierle, O .
CHEMOSPHERE, 1998, 37 (9-12) :2013-2020