Strong coupling between localized plasmons and organic excitons in metal nanovoids

被引:262
作者
Sugawara, Y. [1 ]
Kelf, T. A.
Baumberg, J. J.
Abdelsalam, M. E.
Bartlett, P. N.
机构
[1] Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England
[2] Univ Southampton, Sch Chem, Southampton SO17 1BJ, Hants, England
关键词
D O I
10.1103/PhysRevLett.97.266808
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Hybrid emitting exciton-plasmonic composites are constructed by coating arrays of spherical nanovoids embedded in a gold film with organic semiconducting molecular J-aggregate films. In such plasmonic crystals, localized plasmons confined inside the voids can be excited. We report the first observation of polaritonic spectral narrowing and strong coupling between localized plasmons and J-aggregate excitons with Rabi splittings of 230 meV at room temperature.
引用
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页数:4
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共 23 条
[1]   Preparation of arrays of isolated spherical cavities by self-assembly of polystyrene spheres on self-assembled pre-patterned macroporous films [J].
Abdelsalam, ME ;
Bartlett, PN ;
Baumberg, JJ ;
Coyle, S .
ADVANCED MATERIALS, 2004, 16 (01) :90-+
[2]   Enhancement and quenching of single-molecule fluorescence [J].
Anger, P ;
Bharadwaj, P ;
Novotny, L .
PHYSICAL REVIEW LETTERS, 2006, 96 (11)
[3]  
[Anonymous], SEMICOND SCI TECHNOL
[4]   Angle-resolved surface-enhanced Raman scattering on metallic nanostructured plasmonic crystals [J].
Baumberg, JJ ;
Kelf, TA ;
Sugawara, Y ;
Cintra, S ;
Abdelsalam, ME ;
Bartlett, PN ;
Russell, AE .
NANO LETTERS, 2005, 5 (11) :2262-2267
[5]   Strong coupling between surface plasmons and excitons in an organic semiconductor [J].
Bellessa, J ;
Bonnand, C ;
Plenet, JC ;
Mugnier, J .
PHYSICAL REVIEW LETTERS, 2004, 93 (03) :036404-1
[6]   Confined plasmons in metallic nanocavities [J].
Coyle, S ;
Netti, MC ;
Baumberg, JJ ;
Ghanem, MA ;
Birkin, PR ;
Bartlett, PN ;
Whittaker, DM .
PHYSICAL REVIEW LETTERS, 2001, 87 (17) :176801-176801
[7]   Strong coupling between surface plasmon-polaritons and organic molecules in subwavelength hole arrays [J].
Dintinger, J ;
Klein, S ;
Bustos, F ;
Barnes, WL ;
Ebbesen, TW .
PHYSICAL REVIEW B, 2005, 71 (03)
[8]   Strong exciton-photon coupling in a length tunable optical microcavity with J-aggregate dye heterostructures -: art. no. 041110 [J].
Finlayson, CE ;
Prakash, GV ;
Baumberg, JJ .
APPLIED PHYSICS LETTERS, 2005, 86 (04) :041110-1
[9]   Emission through one of two metal electrodes of an organic light-emitting diode via surface-plasmon cross coupling [J].
Gifford, DK ;
Hall, DG .
APPLIED PHYSICS LETTERS, 2002, 81 (23) :4315-4317
[10]   Strong exciton-photon coupling in a low-Q all-metal mirror microcavity [J].
Hobson, PA ;
Barnes, WL ;
Lidzey, DG ;
Gehring, GA ;
Whittaker, DM ;
Skolnick, MS ;
Walker, S .
APPLIED PHYSICS LETTERS, 2002, 81 (19) :3519-3521