共 24 条
Dynamic electrochemical experiments on hydrogenases
被引:19
作者:

Armstrong, Fraser A.
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Oxford, Inorgan Chem Lab, Dept Chem, Oxford OX1 3QR, England Univ Oxford, Inorgan Chem Lab, Dept Chem, Oxford OX1 3QR, England
机构:
[1] Univ Oxford, Inorgan Chem Lab, Dept Chem, Oxford OX1 3QR, England
基金:
英国工程与自然科学研究理事会;
英国生物技术与生命科学研究理事会;
关键词:
Hydrogen;
Hydrogenase;
Photosynthesis;
Electrochemistry;
H-2;
O-2;
UNREADY;
READY;
INTERCONVERSIONS;
INACTIVATION;
DIFFERENCE;
ACTIVATION;
OXIDATION;
STATES;
D O I:
10.1007/s11120-009-9428-0
中图分类号:
Q94 [植物学];
学科分类号:
071001 ;
摘要:
A powerful approach for studying hydrogenases, applying a suite of dynamic electrochemical techniques known as protein film electrochemistry, is trailblazing fresh discoveries and providing a wealth of quantitative data on these complex enzymes. The information now stemming from experiments on tiny quantities of hydrogenases ranges from their kinetics and catalytic bias (a preference to operate in H-2 oxidation vs. H-2 production) to wide differences in the ways they react with oxygen and other inhibitors. Tolerance of hydrogenase catalysis to oxygen is essential if organisms are to be exploited for photosynthetic hydrogen production, and is crucial in enabling aerobes to use trace H-2 as an energy source. Experiments described in this article may be adapted for other complex enzymes.
引用
收藏
页码:541 / 550
页数:10
相关论文
共 24 条
[1]
Dynamic electrochemical investigations of hydrogen oxidation and production by enzymes and implications for future technology
[J].
Armstrong, Fraser A.
;
Belsey, Natalie A.
;
Cracknell, James A.
;
Goldet, Gabrielle
;
Parkin, Alison
;
Reisner, Erwin
;
Vincent, Kylie A.
;
Wait, Annemarie F.
.
CHEMICAL SOCIETY REVIEWS,
2009, 38 (01)
:36-51

Armstrong, Fraser A.
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England

Belsey, Natalie A.
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England

Cracknell, James A.
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England

Goldet, Gabrielle
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England

Parkin, Alison
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England

Reisner, Erwin
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England

Vincent, Kylie A.
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England

Wait, Annemarie F.
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England
[2]
Finding gas diffusion pathways in proteins:: Application to O2 and H2 transport in Cpl [FeFe]-hydrogenase and the role of packing defects
[J].
Cohen, J
;
Kim, K
;
King, P
;
Seibert, M
;
Schulten, K
.
STRUCTURE,
2005, 13 (09)
:1321-1329

Cohen, J
论文数: 0 引用数: 0
h-index: 0
机构: Univ Illinois, Dept Phys, Urbana, IL 61801 USA

Kim, K
论文数: 0 引用数: 0
h-index: 0
机构: Univ Illinois, Dept Phys, Urbana, IL 61801 USA

King, P
论文数: 0 引用数: 0
h-index: 0
机构: Univ Illinois, Dept Phys, Urbana, IL 61801 USA

Seibert, M
论文数: 0 引用数: 0
h-index: 0
机构: Univ Illinois, Dept Phys, Urbana, IL 61801 USA

Schulten, K
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Illinois, Dept Phys, Urbana, IL 61801 USA Univ Illinois, Dept Phys, Urbana, IL 61801 USA
[3]
Enzymatic oxidation of H2 in atmospheric O2:: The electrochemistry of energy generation from trace H2 by aerobic microorganisms
[J].
Cracknell, James A.
;
Vincent, Kylie A.
;
Ludwig, Marcus
;
Lenz, Oliver
;
Friedrich, Baerbel
;
Armstrong, Fraser A.
.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,
2008, 130 (02)
:424-+

Cracknell, James A.
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Oxford, Inorgan Chem Lab, Oxford OX1 3QR, England Univ Oxford, Inorgan Chem Lab, Oxford OX1 3QR, England

Vincent, Kylie A.
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Oxford, Inorgan Chem Lab, Oxford OX1 3QR, England Univ Oxford, Inorgan Chem Lab, Oxford OX1 3QR, England

Ludwig, Marcus
论文数: 0 引用数: 0
h-index: 0
机构:
Humboldt Univ, Inst Biol Mikrobiol, D-10115 Berlin, Germany Univ Oxford, Inorgan Chem Lab, Oxford OX1 3QR, England

Lenz, Oliver
论文数: 0 引用数: 0
h-index: 0
机构:
Humboldt Univ, Inst Biol Mikrobiol, D-10115 Berlin, Germany Univ Oxford, Inorgan Chem Lab, Oxford OX1 3QR, England

Friedrich, Baerbel
论文数: 0 引用数: 0
h-index: 0
机构:
Humboldt Univ, Inst Biol Mikrobiol, D-10115 Berlin, Germany Univ Oxford, Inorgan Chem Lab, Oxford OX1 3QR, England

Armstrong, Fraser A.
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Oxford, Inorgan Chem Lab, Oxford OX1 3QR, England Univ Oxford, Inorgan Chem Lab, Oxford OX1 3QR, England
[4]
Structure/function relationships of [NiFe]- and [FeFe]-hydrogenases
[J].
Fontecilla-Camps, Juan C.
;
Volbeda, Anne
;
Cavazza, Christine
;
Nicolet, Yvain
.
CHEMICAL REVIEWS,
2007, 107 (10)
:4273-4303

Fontecilla-Camps, Juan C.
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Grenoble 1, CNRS, CEA,Lab Cristallog & Cristallogenese Proteines, Inst Biol Struct J P Ebel, F-38027 Grenoble 1, France Univ Grenoble 1, CNRS, CEA,Lab Cristallog & Cristallogenese Proteines, Inst Biol Struct J P Ebel, F-38027 Grenoble 1, France

Volbeda, Anne
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Grenoble 1, CNRS, CEA,Lab Cristallog & Cristallogenese Proteines, Inst Biol Struct J P Ebel, F-38027 Grenoble 1, France Univ Grenoble 1, CNRS, CEA,Lab Cristallog & Cristallogenese Proteines, Inst Biol Struct J P Ebel, F-38027 Grenoble 1, France

Cavazza, Christine
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Grenoble 1, CNRS, CEA,Lab Cristallog & Cristallogenese Proteines, Inst Biol Struct J P Ebel, F-38027 Grenoble 1, France Univ Grenoble 1, CNRS, CEA,Lab Cristallog & Cristallogenese Proteines, Inst Biol Struct J P Ebel, F-38027 Grenoble 1, France

Nicolet, Yvain
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Grenoble 1, CNRS, CEA,Lab Cristallog & Cristallogenese Proteines, Inst Biol Struct J P Ebel, F-38027 Grenoble 1, France Univ Grenoble 1, CNRS, CEA,Lab Cristallog & Cristallogenese Proteines, Inst Biol Struct J P Ebel, F-38027 Grenoble 1, France
[5]
Hydrogenases and hydrogen photoproduction in oxygenic photosynthetic organisms
[J].
Ghirardi, Maria L.
;
Posewitz, Matthew C.
;
Maness, Pin-Ching
;
Dubini, Alexandra
;
Yu, Jianping
;
Seibert, Michael
.
ANNUAL REVIEW OF PLANT BIOLOGY,
2007, 58
:71-91

Ghirardi, Maria L.
论文数: 0 引用数: 0
h-index: 0
机构:
Natl Renewable Energy Lab, Golden, CO 80401 USA Natl Renewable Energy Lab, Golden, CO 80401 USA

Posewitz, Matthew C.
论文数: 0 引用数: 0
h-index: 0
机构: Natl Renewable Energy Lab, Golden, CO 80401 USA

Maness, Pin-Ching
论文数: 0 引用数: 0
h-index: 0
机构: Natl Renewable Energy Lab, Golden, CO 80401 USA

Dubini, Alexandra
论文数: 0 引用数: 0
h-index: 0
机构: Natl Renewable Energy Lab, Golden, CO 80401 USA

Yu, Jianping
论文数: 0 引用数: 0
h-index: 0
机构: Natl Renewable Energy Lab, Golden, CO 80401 USA

Seibert, Michael
论文数: 0 引用数: 0
h-index: 0
机构: Natl Renewable Energy Lab, Golden, CO 80401 USA
[6]
Hydrogen production under aerobic conditions by membrane-bound hydrogenases from Ralstonia species
[J].
Goldet, Gabrielle
;
Wait, Annemarie F.
;
Cracknell, James A.
;
Vincent, Kylie A.
;
Ludwig, Marcus
;
Lenz, Oliver
;
Friedrich, Baerbel
;
Armstrong, Fraser A.
.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,
2008, 130 (33)
:11106-11113

Goldet, Gabrielle
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England

Wait, Annemarie F.
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England

Cracknell, James A.
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England

Vincent, Kylie A.
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England

Ludwig, Marcus
论文数: 0 引用数: 0
h-index: 0
机构:
Humboldt Univ, Inst Biol Mikrobiol, D-10115 Berlin, Germany Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England

Lenz, Oliver
论文数: 0 引用数: 0
h-index: 0
机构:
Humboldt Univ, Inst Biol Mikrobiol, D-10115 Berlin, Germany Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England

Friedrich, Baerbel
论文数: 0 引用数: 0
h-index: 0
机构:
Humboldt Univ, Inst Biol Mikrobiol, D-10115 Berlin, Germany Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England

Armstrong, Fraser A.
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England
[7]
[FeFe]-Hydrogenase-Catalyzed H2 production in a photoelectrochemical biofuel cell
[J].
Hambourger, Michael
;
Gervaldo, Miguel
;
Svedruzic, Drazenka
;
King, Paul W.
;
Gust, Devens
;
Ghirardi, Maria
;
Moore, Ana L.
;
Moore, Thomas A.
.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,
2008, 130 (06)
:2015-2022

Hambourger, Michael
论文数: 0 引用数: 0
h-index: 0
机构:
Arizona State Univ, Ctr Bioenergy & Photosysnth, Tempe, AZ 85287 USA
Arizona State Univ, Dept Chem & Biochem, Tempe, AZ 85287 USA Natl Renewable Energy Lab, Chem & Biosci Ctr, Golden, CO 80401 USA

论文数: 引用数:
h-index:
机构:

Svedruzic, Drazenka
论文数: 0 引用数: 0
h-index: 0
机构:
Natl Renewable Energy Lab, Chem & Biosci Ctr, Golden, CO 80401 USA Natl Renewable Energy Lab, Chem & Biosci Ctr, Golden, CO 80401 USA

King, Paul W.
论文数: 0 引用数: 0
h-index: 0
机构:
Natl Renewable Energy Lab, Chem & Biosci Ctr, Golden, CO 80401 USA Natl Renewable Energy Lab, Chem & Biosci Ctr, Golden, CO 80401 USA

Gust, Devens
论文数: 0 引用数: 0
h-index: 0
机构:
Arizona State Univ, Ctr Bioenergy & Photosysnth, Tempe, AZ 85287 USA
Arizona State Univ, Dept Chem & Biochem, Tempe, AZ 85287 USA Natl Renewable Energy Lab, Chem & Biosci Ctr, Golden, CO 80401 USA

Ghirardi, Maria
论文数: 0 引用数: 0
h-index: 0
机构:
Natl Renewable Energy Lab, Chem & Biosci Ctr, Golden, CO 80401 USA Natl Renewable Energy Lab, Chem & Biosci Ctr, Golden, CO 80401 USA

Moore, Ana L.
论文数: 0 引用数: 0
h-index: 0
机构:
Arizona State Univ, Ctr Bioenergy & Photosysnth, Tempe, AZ 85287 USA
Arizona State Univ, Dept Chem & Biochem, Tempe, AZ 85287 USA Natl Renewable Energy Lab, Chem & Biosci Ctr, Golden, CO 80401 USA

论文数: 引用数:
h-index:
机构:
[8]
Direct comparison of the electrocatalytic oxidation of hydrogen by an enzyme and a platinum catalyst
[J].
Jones, AK
;
Sillery, E
;
Albracht, SPJ
;
Armstrong, FA
.
CHEMICAL COMMUNICATIONS,
2002, (08)
:866-867

Jones, AK
论文数: 0 引用数: 0
h-index: 0
机构: Univ Oxford, Dept Chem, Oxford OX1 3QR, England

Sillery, E
论文数: 0 引用数: 0
h-index: 0
机构: Univ Oxford, Dept Chem, Oxford OX1 3QR, England

Albracht, SPJ
论文数: 0 引用数: 0
h-index: 0
机构: Univ Oxford, Dept Chem, Oxford OX1 3QR, England

Armstrong, FA
论文数: 0 引用数: 0
h-index: 0
机构: Univ Oxford, Dept Chem, Oxford OX1 3QR, England
[9]
The mechanism of activation of a [NiFe]-hydrogenase by electrons, hydrogen, and carbon monoxide
[J].
Lamle, SE
;
Albracht, SPJ
;
Armstrong, FA
.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,
2005, 127 (18)
:6595-6604

Lamle, SE
论文数: 0 引用数: 0
h-index: 0
机构: Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England

Albracht, SPJ
论文数: 0 引用数: 0
h-index: 0
机构: Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England

Armstrong, FA
论文数: 0 引用数: 0
h-index: 0
机构: Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England
[10]
Electrochemical potential-step investigations of the aerobic interconversions of [NiFe]-hydrogenase from Allochromatium vinosum:: Insights into the puzzling difference between unready and ready oxidized inactive states
[J].
Lamle, SE
;
Albracht, SPJ
;
Armstrong, FA
.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,
2004, 126 (45)
:14899-14909

Lamle, SE
论文数: 0 引用数: 0
h-index: 0
机构: Univ Oxford, Inorgan Chem Lab, Dept Chem, Oxford OX1 3QR, England

Albracht, SPJ
论文数: 0 引用数: 0
h-index: 0
机构: Univ Oxford, Inorgan Chem Lab, Dept Chem, Oxford OX1 3QR, England

Armstrong, FA
论文数: 0 引用数: 0
h-index: 0
机构: Univ Oxford, Inorgan Chem Lab, Dept Chem, Oxford OX1 3QR, England