Field-effect transistors based on a benzothiadiazole-cyclopentadithiophene copolymer

被引：459

作者：

Zhang, Ming ^{[1
]}

Tsao, Hoi Nok ^{[1
]}

Pisula, Wojciech ^{[1
]}

Yang, Changduk ^{[1
]}

Mishra, Ashok K. ^{[1
]}

Muellen, Klaus ^{[1
]}

机构：

[1] Max Planck Inst Polymer Res, D-55128 Mainz, Germany

来源：

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY | 2007年 / 129卷 / 12期

关键词：

D O I：

10.1021/ja0683537

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

We present a solution processed organic field-effect transistor based on a benzothiadiazole (BTZ)cyclopentadithiophene (CDT) copolymer with mobilities as high as 0.17 cm(2)/Vs and an on/off ratio of 10(5). This pronounced performance together with the lack of macroscopic order in the thin film makes this conjugated copolymer an attractive candidate for low-cost organic electronics due to its facile processing.

引用

收藏

页码：3472 / +

页数：3

相关论文

共 21 条

[1] Cyclopentadithiophene based electroactive materials [J].

Coppo, P ;

Turner, ML .

JOURNAL OF MATERIALS CHEMISTRY, 2005, 15 (11) :1123-1133

[2] Synthetic routes to solution-processable polycyclopentadithiophenes [J].

Coppo, P ;

Cupertino, DC ;

Yeates, SG ;

Turner, ML .

MACROMOLECULES, 2003, 36 (08) :2705-2711

[3]

Dimitrakopoulos CD, 2002, ADV MATER, V14, P99, DOI 10.1002/1521-4095(20020116)14:2<99::AID-ADMA99>3.0.CO

[4]

2-9

[5] Regiosymmetric poly (dialkylphenylenedioxythiophene)s:: Electron-rich, stackable π-conjugated nanoribbons [J].

Grenier, Christophe R. G. ;

Pisula, Wojciech ;

Joncheray, Thomas J. ;

Muellen, Klaus ;

Reynolds, John R. .

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2007, 46 (05) :714-717

[6] Plastic transistors in active-matrix displays - The handling of grey levels by these large displays paves the way for electronic paper. [J].

Huitema, HEA ;

Gelinck, GH ;

van der Putten, JBPH ;

Kuijk, KE ;

Hart, CM ;

Cantatore, E ;

Herwig, PT ;

van Breemen, AJJM ;

de Leeuw, DM .

NATURE, 2001, 414 (6864) :599-599

[7] A strong regioregularity effect in self-organizing conjugated polymer films and high-efficiency polythiophene: fullerene solar cells [J].

Kim, Y ;

Cook, S ;

Tuladhar, SM ;

Choulis, SA ;

Nelson, J ;

Durrant, JR ;

Bradley, DDC ;

Giles, M ;

Mcculloch, I ;

Ha, CS ;

Ree, M .

NATURE MATERIALS, 2006, 5 (03) :197-203

[8] Polyindolo[3,2-b]carbazoles:: A new class of p-channel semiconductor polymers for organic thin-film transistors [J].

Li, Yuning ;

Wu, Yiliang ;

Ong, Beng S. .

MACROMOLECULES, 2006, 39 (19) :6521-6527

[9] Poly(2,5-bis(2-thienyl)-3,6-dialkylthieno[3,2-b]thiophene)s-high-mobility semiconductors for thin-film transistors [J].

Li, Yuning ;

Wu, Yiliang ;

Liu, Ping ;

Birau, Maria ;

Pan, Hualong ;

Ong, Beng S. .

ADVANCED MATERIALS, 2006, 18 (22) :3029-+

[10] Liquid-crystalline semiconducting polymers with high charge-carrier mobility [J].

Mcculloch, I ;

Heeney, M ;

Bailey, C ;

Genevicius, K ;

Macdonald, I ;

Shkunov, M ;

Sparrowe, D ;

Tierney, S ;

Wagner, R ;

Zhang, WM ;

Chabinyc, ML ;

Kline, RJ ;

Mcgehee, MD ;

Toney, MF .

NATURE MATERIALS, 2006, 5 (04) :328-333