Wigner spectrogram representations of heterodyne-detected four-wave-mixing and fluorescence up-conversion

被引:39
作者
Mukamel, S
机构
[1] Department of Chemistry, University of Rochester, Rochester
关键词
D O I
10.1063/1.474791
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Gated spontaneous emission and four-wave-mixing signals ar expressed using a mixed time-frequency representation of the fields (Wigner spectrograms) and of the material response functions. Well-separated and overlapping pulses are described using two-sided (noncausal) and one-sided (causal) spectrograms, respectively. Pump-probe and fluorescence spectra are recast in an anologous form which facilitates the direct comparison of the underlying microscopic dynamics. (C) 1997 American Institute of Physics.
引用
收藏
页码:4165 / 4171
页数:7
相关论文
共 61 条
[1]   DETECTION, ESTIMATION, AND CLASSIFICATION WITH SPECTROGRAMS [J].
ALTES, RA .
JOURNAL OF THE ACOUSTICAL SOCIETY OF AMERICA, 1980, 67 (04) :1232-1246
[2]  
Barbara P. F., 1990, ADV PHOTOCHEM, V15, P1, DOI [DOI 10.1002/9780470133453.CHL, DOI 10.1103/PhysRevLett.88.158101]
[3]   INSTANTANEOUS FREQUENCY DYNAMICS OF COHERENT WAVE MIXING IN SEMICONDUCTOR QUANTUM-WELLS [J].
BIGOT, JY ;
MYCEK, MA ;
WEISS, S ;
ULBRICH, RG ;
CHEMLA, DS .
PHYSICAL REVIEW LETTERS, 1993, 70 (21) :3307-3310
[4]  
Bloembergen N., 1965, NONLINEAR OPTICS
[5]   THE TIME-DEPENDENT PHYSICAL SPECTRUM OF LIGHT AND THE WIGNER DISTRIBUTION FUNCTION [J].
BRENNER, KH ;
WODKIEWICZ, K .
OPTICS COMMUNICATIONS, 1982, 43 (02) :103-106
[6]  
Butcher P. N., 1990, ELEMENT NONLINEAR OP
[7]  
CHEMLA DS, 1992, PHYS REV B, V69, P3631
[8]  
CHEMLA DS, 1994, PHYS REV A, V50, P8449
[9]   ULTRAFAST SOLVENT DYNAMICS - CONNECTION BETWEEN TIME RESOLVED FLUORESCENCE AND OPTICAL KERR MEASUREMENTS [J].
CHO, MH ;
ROSENTHAL, SJ ;
SCHERER, NF ;
ZIEGLER, LD ;
FLEMING, GR .
JOURNAL OF CHEMICAL PHYSICS, 1992, 96 (07) :5033-5038
[10]   TIME FREQUENCY-DISTRIBUTIONS - A REVIEW [J].
COHEN, L .
PROCEEDINGS OF THE IEEE, 1989, 77 (07) :941-981