Wigner spectrogram representations of heterodyne-detected four-wave-mixing and fluorescence up-conversion

被引:39
作者
Mukamel, S
机构
[1] Department of Chemistry, University of Rochester, Rochester
关键词
D O I
10.1063/1.474791
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Gated spontaneous emission and four-wave-mixing signals ar expressed using a mixed time-frequency representation of the fields (Wigner spectrograms) and of the material response functions. Well-separated and overlapping pulses are described using two-sided (noncausal) and one-sided (causal) spectrograms, respectively. Pump-probe and fluorescence spectra are recast in an anologous form which facilitates the direct comparison of the underlying microscopic dynamics. (C) 1997 American Institute of Physics.
引用
收藏
页码:4165 / 4171
页数:7
相关论文
共 61 条
[31]  
Mandel L., 1995, Optical Coherence and Quantum Optics
[32]   DIRECT OBSERVATION OF THE FEMTOSECOND EXCITED-STATE CIS-TRANS ISOMERIZATION IN BACTERIORHODOPSIN [J].
MATHIES, RA ;
CRUZ, CHB ;
POLLARD, WT ;
SHANK, CV .
SCIENCE, 1988, 240 (4853) :777-779
[33]   Femtosecond spectroscopic signatures of electronic correlations in conjugated polyenes and semiconductor nanostructures [J].
Meier, T ;
Mukamel, S .
PHYSICAL REVIEW LETTERS, 1996, 77 (16) :3471-3474
[34]  
MEIER T, IN PRESS J CHEM PHYS
[36]   Wigner spectrograms for femtosecond pulse-shaped heterodyne and autocorrelation measurements [J].
Mukamel, S ;
CiordasCiurdariu, C ;
Khidekel, V .
IEEE JOURNAL OF QUANTUM ELECTRONICS, 1996, 32 (08) :1278-1288
[38]   Time-frequency and coordinate-momentum Wigner wavepackets in nonlinear spectroscopy [J].
Mukamel, S ;
CiordasCiurdariu, C ;
Khidekel, V .
CHEMICAL REACTIONS AND THEIR CONTROL ON THE FEMTOSECOND TIME SCALE XXTH SOLVAY CONFERENCE ON CHEMISTRY, 1997, 101 :345-371
[39]  
MUKAMEL S, 1997, NOBEL S, V101
[40]  
Mukamel S., 1995, Principles of Nonlinear Optical Spectroscopy