AMS measurement of environmental U-236 preliminary results and perspectives

被引:49
作者
Zhao, XL [1 ]
Kilius, LR [1 ]
Litherland, AE [1 ]
Beasley, T [1 ]
机构
[1] US DOE,NEW YORK,NY 10014
关键词
AMS; heavy element; actinide; U-236;
D O I
10.1016/S0168-583X(96)01034-8
中图分类号
TH7 [仪器、仪表];
学科分类号
0804 ; 080401 ; 081102 ;
摘要
U-236 is a 23.4 Ma half-life radioactive isotope whose natural global abundance is expected to be overwhelmed in many places by its production and release during nuclear power generation. The detection of excess U-236 in the environment is therefore a method of monitoring the presence of activated uranium. However, U-236 has not been widely used for environmental studies due to the difficulties of measuring it at low levels with standard cu-spectrometry or thermal ionization mass spectrometry. In principle, accelerator mass spectrometry can overcome some of the difficulties encountered in the traditional methods, making it possible to detect U-236 at very low levels so that a large range of environmental samples can be analyzed. In this paper, we report some preliminary results of the U-236 measurements of four water samples from the US Idaho Chemical Processing Plant. Limitations with our current AMS system and the perspectives for considerable improvements will be discussed.
引用
收藏
页码:297 / 300
页数:4
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