Ising versus XY Anisotropy in Frustrated R2Ti2O7 Compounds as "Seen'' by Polarized Neutrons

被引:100
作者
Cao, H. [1 ]
Gukasov, A. [1 ]
Mirebeau, I. [1 ]
Bonville, P. [2 ]
Decorse, C. [3 ]
Dhalenne, G. [3 ]
机构
[1] CE Saclay, CEA, CNRS, Lab Leon Brillouin, F-91191 Gif Sur Yvette, France
[2] CE Saclay, CEA, CNRS, Serv Phys Etat Condense, F-91191 Gif Sur Yvette, France
[3] Univ Paris 11, ICMMO, Lab Physicochim Etat Solide, F-91405 Orsay, France
关键词
PYROCHLORE ANTIFERROMAGNET TB2TI2O7; SITE SUSCEPTIBILITY TENSORS; CRYSTAL-FIELD; SPIN ICE; DIFFRACTION; YB2TI2O7; HO2TI2O7; STATE;
D O I
10.1103/PhysRevLett.103.056402
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We studied the field induced magnetic order in R2Ti2O7 pyrochlore compounds with either uniaxial (R = Ho, Tb) or planar (R = Er, Yb) anisotropy, by polarized neutron diffraction. The determination of the local susceptibility tensor {chi(parallel to), chi(perpendicular to)} provides a universal description of the field induced structures in the paramagnetic phase (2-270 K), whatever the field value (1-7 T) and direction. Comparison of the thermal variations of chi(parallel to) and chi(perpendicular to) with calculations using the rare earth crystal field shows that exchange and dipolar interactions must be taken into account. We determine the molecular field tensor in each case and show that it can be strongly anisotropic.
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页数:4
相关论文
共 31 条
[1]   HEAT-CAPACITY MEASUREMENTS ON RARE-EARTH DOUBLE OXIDES R2M2O7 [J].
BLOTE, HWJ ;
WIELINGA, RF ;
HUISKAMP, WJ .
PHYSICA, 1969, 43 (04) :549-&
[2]   Spin ice state in frustrated magnetic pyrochlore materials [J].
Bramwell, ST ;
Gingras, MJP .
SCIENCE, 2001, 294 (5546) :1495-1501
[3]   Spin correlations in Ho2Ti2O7:: A dipolar spin ice system -: art. no. 047205 [J].
Bramwell, ST ;
Harris, MJ ;
den Hertog, BC ;
Gingras, MJP ;
Gardner, JS ;
McMorrow, DF ;
Wildes, AR ;
Cornelius, AL ;
Champion, JDM ;
Melko, RG ;
Fennell, T .
PHYSICAL REVIEW LETTERS, 2001, 87 (04) :47205-1
[4]  
BROWN PJ, 1993, CCSLRAL93009, P52409
[5]   Field-Induced Spin-Ice-Like Orders in Spin Liquid Tb2Ti2O7 [J].
Cao, H. ;
Gukasov, A. ;
Mirebeau, I. ;
Bonville, P. ;
Dhalenne, G. .
PHYSICAL REVIEW LETTERS, 2008, 101 (19)
[6]   Er2Ti2O7:: Evidence of quantum order by disorder in a frustrated antiferromagnet -: art. no. 020401 [J].
Champion, JDM ;
Harris, MJ ;
Holdsworth, PCW ;
Wills, AS ;
Balakrishnan, G ;
Bramwell, ST ;
Cizmár, E ;
Fennell, T ;
Gardner, JS ;
Lago, J ;
McMorrow, DF ;
Orendác, M ;
Orendácová, A ;
Paul, DM ;
Smith, RI ;
Telling, MTF ;
Wildes, A .
PHYSICAL REVIEW B, 2003, 68 (02)
[7]   Dipolar interactions and origin of spin ice in Ising pyrochlore magnets [J].
den Hertog, BC ;
Gingras, MJP .
PHYSICAL REVIEW LETTERS, 2000, 84 (15) :3430-3433
[8]   Spin-spin correlations in Yb2Ti2O7:: A polarized neutron scattering study -: art. no. 180404 [J].
Gardner, JS ;
Ehlers, G ;
Rosov, N ;
Erwin, RW ;
Petrovic, C .
PHYSICAL REVIEW B, 2004, 70 (18) :1-4
[9]   Cooperative paramagnetism in the geometrically frustrated pyrochlore antiferromagnet Tb2Ti2O7 [J].
Gardner, JS ;
Dunsiger, SR ;
Gaulin, BD ;
Gingras, MJP ;
Greedan, JE ;
Kiefl, RF ;
Lumsden, MD ;
MacFarlane, WA ;
Raju, NP ;
Sonier, JE ;
Swainson, I ;
Tun, Z .
PHYSICAL REVIEW LETTERS, 1999, 82 (05) :1012-1015
[10]   Thermodynamic and single-ion properties of Tb3+ within the collective paramagnetic-spin liquid state of the frustrated pyrochlore antiferromagnet Tb2Ti2O7 [J].
Gingras, MJP ;
den Hertog, BC ;
Faucher, M ;
Gardner, JS ;
Dunsiger, SR ;
Chang, LJ ;
Gaulin, BD ;
Raju, NP ;
Greedan, JE .
PHYSICAL REVIEW B, 2000, 62 (10) :6496-6511