Comparative measures of single-wall carbon nanotube dispersion

被引：76

作者：

Fagan, J. A. ^{[1
]}

Landi, B. J.

Mandelbaum, I.

Simpson, J. R.

Bajpai, V.

Bauer, B. J.

Migler, K.

Walker, A. R. Hight

Raffaelle, R.

Hobbie, E. K.

机构：

[1] Natl Inst Stand & Technol, Div Polymers, Gaithersburg, MD 20899 USA

[2] Natl Inst Stand & Technol, Phys Lab, Gaithersburg, MD 20899 USA

[3] Rochester Inst Technol, NanoPower Res Labs, Rochester, NY 14623 USA

来源：

JOURNAL OF PHYSICAL CHEMISTRY B | 2006年 / 110卷 / 47期

关键词：

ANGLE NEUTRON-SCATTERING; RAMAN-SPECTROSCOPY; SUSPENSIONS;

D O I：

10.1021/jp0647434

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Model composites of DNA-wrapped single-wall carbon nanotubes in poly(acrylic acid) are used to evaluate metrics of nanotube dispersion. By varying the pH of the precursor solutions, we introduce a controlled deviation from ideal behavior. On the basis of small-angle neutron scattering, changes in near-infrared fluorescence intensity are strongly correlated with dispersion, while optical absorption spectroscopy and resonant Raman scattering are less definitive. Our results represent the first systematic comparison of currently accepted measures of nanotube dispersion.

引用

页码：23801 / 23805

页数：5

共 25 条

[11] Structure of semidilute single-wall carbon nanotube suspensions and gels [J].

Hough, LA ;

Islam, MF ;

Hammouda, B ;

Yodh, AG ;

Heiney, PA .

NANO LETTERS, 2006, 6 (02) :313-317

[12]

Jones M, 2005, PHYS REV B, V71, DOI 10.1103/PhysRevB.71.115426

[13] Effects of alkyl amide solvents on the dispersion of single-wall carbon nanotubes [J].

Landi, BJ ;

Ruf, HJ ;

Worman, JJ ;

Raffaelle, RP .

JOURNAL OF PHYSICAL CHEMISTRY B, 2004, 108 (44) :17089-17095

[14] Dispersion of single-walled carbon nanotube bundles in nonaqueous solution [J].

Maeda, Y ;

Kimura, S ;

Hirashima, Y ;

Kanda, M ;

Lian, YF ;

Wakahara, T ;

Akasaka, T ;

Hasegawa, T ;

Tokumoto, H ;

Shimizu, T ;

Kataura, H ;

Miyauchi, Y ;

Maruyama, S ;

Kobayashi, K ;

Nagase, S .

JOURNAL OF PHYSICAL CHEMISTRY B, 2004, 108 (48) :18395-18397

[15] Method for measuring the Raman gain tensor in optical fibers [J].

Mandelbaum, I ;

Bolshtyansky, M ;

Heinz, TF ;

Walker, ARH .

JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS, 2006, 23 (04) :621-627

[16] Band gap fluorescence from individual single-walled carbon nanotubes [J].

O'Connell, MJ ;

Bachilo, SM ;

Huffman, CB ;

Moore, VC ;

Strano, MS ;

Haroz, EH ;

Rialon, KL ;

Boul, PJ ;

Noon, WH ;

Kittrell, C ;

Ma, JP ;

Hauge, RH ;

Weisman, RB ;

Smalley, RE .

SCIENCE, 2002, 297 (5581) :593-596

[17] Near-infrared resonance Raman excitation profile studies of single-walled carbon nanotube intertube interactions: A direct comparison of bundled and individually dispersed HiPco nanotubes [J].

O'Connell, MJ ;

Sivaram, S ;

Doorn, SK .

PHYSICAL REVIEW B, 2004, 69 (23) :235415-1

[18] Neutron scattering studies of the structure and dynamics of nanobundles of single-wall carbon nanotubes [J].

Rols, S ;

Anglaret, E ;

Sauvajol, JL ;

Coddens, G ;

Dianoux, AJ .

APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING, 1999, 69 (06) :591-596

[19] Structure and dispersion of carbon nanotubes [J].

Schaefer, D ;

Brown, JM ;

Anderson, DP ;

Zhao, J ;

Chokalingam, K ;

Tomlin, D ;

Ilavsky, J .

JOURNAL OF APPLIED CRYSTALLOGRAPHY, 2003, 36 :553-557

[20] Morphology of dispersed carbon single-walled nanotubes [J].

Schaefer, DW ;

Zhao, J ;

Brown, JM ;

Anderson, DP ;

Tomlin, DW .

CHEMICAL PHYSICS LETTERS, 2003, 375 (3-4) :369-375

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