Fluorescence signals of core-shell quantum dots enhanced by single crystalline gold caps on silicon nanowires

被引:6
作者
Christiansen, S. H. [1 ,2 ]
Chou, J. W. [1 ,3 ]
Becker, M. [1 ,2 ]
Sivakov, V. [1 ,2 ]
Ehrhold, K. [1 ]
Berger, A. [1 ,2 ]
Chou, W. C. [3 ]
Chuu, D. S. [3 ]
Goesele, U. [1 ]
机构
[1] Max Planck Inst Microstruct Phys, D-06120 Halle, Germany
[2] IPHT, D-07745 Jena, Germany
[3] Natl Chiao Tung Univ, Dept Electrophys, Hsinchu 30050, Taiwan
关键词
ELECTRON-BEAM EVAPORATION; RESONANCE ENERGY-TRANSFER; LIQUID-SOLID GROWTH; SEMICONDUCTOR NANOCRYSTALS; SILVER NANOPARTICLES; LUMINESCENCE; INTERBAND; DONORS; MODEL; SIZE;
D O I
10.1088/0957-4484/20/16/165301
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
We use nanoscale (20-300 nm in diameter) single crystalline gold (Au)-caps on silicon nanowires (NWs) grown by the vapor-liquid-solid (VLS) growth mechanism to enhance the fluorescence photoluminescence (PL) signals of highly dilute core/shell CdSeTe/ZnS quantum dots (QDs) in aqueous solution (10(-5) M). For NWs without Au-caps, as they appear, for example, after Au etching in aqua regia or buffered KI/I-2-solution, essentially no fluorescence signal of the same diluted QDs could be observed. Fluorescence PL signals were measured using excitation with a laser wavelength of 633 nm. The signal enhancement by single crystalline, nanoscale Au-caps is discussed and interpreted based on finite element modeling (FEM).
引用
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页数:9
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