Structure, Energy, Synergy, Time-The Fundamentals of Process Intensification

被引:437
作者
Van Gerven, Tom [1 ]
Stankiewicz, Andrzej [1 ]
机构
[1] Delft Univ Technol, Proc & Energy Dept, NL-2628 CA Delft, Netherlands
关键词
GAS-PHASE CATALYSIS; MULTIFUNCTIONAL REACTORS; PHOTOCATALYTIC REACTOR; ORGANIC-SYNTHESIS; MAGNETIC-FIELD; MOLECULES; CHEMISTRY; ORIENTATION; DESIGN; FLOW;
D O I
10.1021/ie801501y
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Process intensification (PI) is commonly seen as one of the most promising development paths for the chemical process industry and one of the most important progress areas for modern chemical engineering. Often illustrated with spectacular examples, process intensification struggles, however, with its definition and interpretation. Instead of narrowing the scientific discussion down to finding a commonly accepted definition of PI, it is more important to determine its position within chemical engineering and to identify its fundamentals. Accordingly, the paper presents a fundamental vision on process intensification. The vision encompasses four approaches in spatial, thermodynamic, functional, and temporal domains, which are used to realize four generic principles of PI. The approaches refer to all scales existing in chemical processes, from molecular to meso- and macroscale, and are illustrated with relevant examples with special attention given to the molecular scale.
引用
收藏
页码:2465 / 2474
页数:10
相关论文
共 104 条
[31]   Patterning of flow and mixing in rotating radial microchannels [J].
Ducrée, J ;
Haeberle, S ;
Brenner, T ;
Glatzel, T ;
Zengerle, R .
MICROFLUIDICS AND NANOFLUIDICS, 2006, 2 (02) :97-105
[32]   Cyclodextrin-based catalysts and molecular reactors [J].
Easton, CJ .
PURE AND APPLIED CHEMISTRY, 2005, 77 (11) :1865-1871
[33]   Thermal pattern formation and process intensification in chemical reaction engineering [J].
Eigenberger, Gerhart ;
Kolios, Grigorios ;
Nieken, Ulrich .
CHEMICAL ENGINEERING SCIENCE, 2007, 62 (18-20) :4825-4841
[34]   Towards a methodology for the systematic analysis and design of efficient chemical processes Part 1. From unit operations to elementary process functions [J].
Freund, Hannsjoerg ;
Sundmacher, Kai .
CHEMICAL ENGINEERING AND PROCESSING-PROCESS INTENSIFICATION, 2008, 47 (12) :2051-2060
[35]   SPATIAL ORIENTATION OF MOLECULES IN STRONG ELECTRIC-FIELDS AND EVIDENCE FOR PENDULAR STATES [J].
FRIEDRICH, B ;
HERSCHBACH, DR .
NATURE, 1991, 353 (6343) :412-414
[36]   Microsecond catalytic partial oxidation of alkanes [J].
Goetsch, DA ;
Schmidt, LD .
SCIENCE, 1996, 271 (5255) :1560-1562
[37]   Cavitational reactors for process intensification of chemical processing applications: A critical review [J].
Gogate, Parag R. .
CHEMICAL ENGINEERING AND PROCESSING-PROCESS INTENSIFICATION, 2008, 47 (04) :515-527
[38]   Sonophotocatalytic reactors for wastewater treatment: A critical review [J].
Gogate, PR ;
Pandit, AB .
AICHE JOURNAL, 2004, 50 (05) :1051-1079
[39]   Enhanced catalyst performance using integrated structured functionalities [J].
Grünewald, M ;
Agar, DW .
CHEMICAL ENGINEERING SCIENCE, 2004, 59 (22-23) :5519-5526
[40]   OPTIMIZATION OF BIFUNCTIONAL CATALYST SYSTEMS [J].
GUNN, DJ .
CHEMICAL ENGINEERING SCIENCE, 1967, 22 (07) :963-&