Gain calibration of a β/γ coincidence spectrometer for automated radioxenon analysis

Detection and measurement of atmospheric radioxenon is an important component of international monitoring systems for nuclear weapons testing. Monitoring stations separate xenon from air and perform isotopic analysis of the radioxenon. In one such radioxenon measurement scheme, the isotopes of interest are identified by coincident spectroscopy of electrons and photons in a beta/gamma coincidence spectrometer (BGCS). The beta spectrometer is a plastic scintillator, manufactured as a cylindrical cell containing the separated xenon sample. This cell is surrounded by the NaI(Tl) gamma spectrometer. We report here the development of a calibration process for the BGCS suitable for use in remote sampling systems. This procedure is based upon gamma-ray Compton scattering, resulting in a true coincident signal in both detectors, generation of electrons over a wide energy range that matches the energy distribution of electrons from radioxenon decay, and a relative insensitivity to source location. In addition to gain calibration, this procedure determines the resolution of the beta detector as a function of energy. (C) 2003 Elsevier B.V. All rights reserved.