Diamonds with a high density of nitrogen-vacancy centers for magnetometry applications

被引:451
作者
Acosta, V. M. [1 ]
Bauch, E. [1 ,2 ]
Ledbetter, M. P. [1 ]
Santori, C. [3 ]
Fu, K. -M. C. [3 ]
Barclay, P. E. [3 ]
Beausoleil, R. G. [3 ]
Linget, H.
Roch, J. F. [4 ]
Treussart, F. [4 ]
Chemerisov, S. [5 ]
Gawlik, W. [6 ]
Budker, D. [1 ,7 ]
机构
[1] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA
[2] Tech Univ Berlin, D-10623 Berlin, Germany
[3] Hewlett Packard Labs, Palo Alto, CA 94304 USA
[4] Ecole Normale Super, CNRS, UMR 8537, Lab Photon Quant & Mol, F-94235 Cachan, France
[5] Argonne Natl Lab, Argonne, IL 60439 USA
[6] Jagiellonian Univ, Inst Phys, Ctr Magnetoopt Res, PL-30059 Krakow, Poland
[7] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Nucl Sci, Berkeley, CA 94720 USA
来源
PHYSICAL REVIEW B | 2009年 / 80卷 / 11期
关键词
PARAMAGNETIC-RESONANCE; INFRARED-ABSORPTION; SYNTHETIC DIAMOND; THRESHOLD ENERGY; DEFECT CENTERS; ELECTRON; SPECTRA; SPIN; DISPLACEMENT; IRRADIATION;
D O I
10.1103/PhysRevB.80.115202
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Nitrogen-vacancy (NV) centers in millimeter-scale diamond samples were produced by irradiation and subsequent annealing under varied conditions. The optical and spin-relaxation properties of these samples were characterized using confocal microscopy, visible and infrared absorption, and optically detected magnetic resonance. The sample with the highest NV(-) concentration, approximately 16 ppm (2.8 x 10(18) cm(-3)), was prepared with no observable traces of neutrally charged vacancy defects. The effective transverse spin-relaxation time for this sample was T(2)* = 118 (48) ns, predominately limited by residual paramagnetic nitrogen which was determined to have a concentration of 49(7) ppm. Under ideal conditions, the shot-noise limited sensitivity is projected to be similar to 150 fT/root Hz for a 100 mu m-scale magnetometer based on this sample. Other samples with NV(-) concentrations from 0.007 to 12 ppm and effective relaxation times ranging from 27 to over 291 ns were prepared and characterized.
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页数:15
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