Complete d-band dispersion relation in sodium cobaltates

被引:63
作者
Qian, D. [1 ]
Wray, L.
Hsieh, D.
Viciu, L.
Cava, R. J.
Luo, J. L.
Wu, D.
Wang, N. L.
Hasan, M. Z.
机构
[1] Princeton Univ, Joseph Henry Labs, Dept Phys, Princeton, NJ 08544 USA
[2] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA
[3] Chinese Acad Sci, Inst Phys, Beijing 100080, Peoples R China
关键词
D O I
10.1103/PhysRevLett.97.186405
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We utilize fine-tuned polarization selection coupled with excitation-energy variation of photoelectron signal to image the complete d-band dispersion relation in sodium cobaltates. A hybridization gap anticrossing is observed along the Brillouin zone corner and the full quasiparticle band is found to emerge as a many-body entity lacking a pure orbital polarization. At low dopings, the quasiparticle bandwidth (Fermion scale, many-body E-F similar to 0.25 eV) is found to be smaller than most known oxide metals. The low-lying density of states is found to be in agreement with bulk-sensitive thermodynamic measurements for nonmagnetic dopings where the 2D Luttinger theorem is also observed to be satisfied.
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页数:4
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