Nd isotopic composition in the central North Pacific

被引:86
作者
Amakawa, Hiroshi [1 ]
Sasaki, Kazunori [2 ]
Ebihara, Mitsuru [2 ]
机构
[1] Univ Tokyo, Ctr Adv Marine Res, Ocean Res Inst, Nakano Ku, Tokyo 1648639, Japan
[2] Tokyo Metropolitan Univ, Fac Sci, Dept Chem, Tokyo 1920397, Japan
关键词
PRECISE DETERMINATION; INTERMEDIATE WATER; NEODYMIUM ISOTOPES; SURFACE WATERS; OCEAN; CIRCULATION; SEAWATER; RATIOS; EVOLUTION; INPUTS;
D O I
10.1016/j.gca.2009.05.058
中图分类号
P3 [地球物理学]; P59 [地球化学];
学科分类号
0708 ; 070902 ;
摘要
Three vertical profiles of seawater concentration and isotopic composition of Nd were determined for the western to central North Pacific Ocean. In the Subarctic oceanic region, at depths greater than 500 m, one vertical profile of Nd isotopic composition was indistinguishable from most previously reported profiles from here. The data indicate a rather homogeneous Nd isotopic composition in the subarctic oceanic region at middle to deep depths (>500 m). Two stations in the subtropical oceanic region exhibited similar Nd isotopic composition profiles to those previously reported. The maxima epsilon(Nd) values at depths of 800-1000 m (epsilon(Nd) = -3.4 to -2.7), which correspond to the North Pacific Intermediate Water (NPIW), are found at both subtropical stations. This implies a ubiquitous distribution of NPIW showing a radiogenic epsilon(Nd) value in the North Pacific. The sub-surface minimum at a depth of similar to 200 m, which indicates the penetration of the North Pacific Tropical Water (NPTW) with an unradiogenic Nd isotopic signal, was observed at one station in the western Pacific. This station had much lower epsilon(Nd) than the central station at depths around 5000 m, suggesting the greater prominence of Antarctic Bottom Water (AABW) in the western Subtropical Pacific than in the central to eastern Subtropical Pacific. Results of a model calculation assuming boundary exchange indicate that the Hawaiian Islands play an important role in supplying radiogenic Nd to the central Pacific, similar to some continental margins. We show that Nd isotopic composition is a versatile tracer for ocean Circulation and the geochemical cycle of Nd in the North Pacific. Further studies oil the distribution of Nd isotopic composition in the Pacific Ocean, including the Southern Pacific, will better elucidate the circulation and geochemical cycle of Nd in the Pacific. (C) 2009 Elsevier Ltd. All rights reserved.
引用
收藏
页码:4705 / 4719
页数:15
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