Magnetic-field-induced condensation of triplons in Han Purple pigment BaCuSi2O6 -: art. no. 087203

被引:249
作者
Jaime, M
Correa, VF
Harrison, N
Batista, CD
Kawashima, N
Kazuma, Y
Jorge, GA
Stern, R
Heinmaa, I
Zvyagin, SA
Sasago, Y
Uchinokura, K
机构
[1] Los Alamos Natl Lab, Natl High Magnet Field Lab, Los Alamos, NM 87545 USA
[2] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA
[3] Tokyo Metropolitan Univ, Dept Phys, Tokyo 1920397, Japan
[4] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina
[5] NICPB, EE-12618 Tallinn, Estonia
[6] Natl Magnet Field Lab, Tallahassee, FL 32310 USA
[7] Univ Tokyo, Dept Appl Phys, Tokyo 1138656, Japan
基金
美国国家科学基金会;
关键词
D O I
10.1103/PhysRevLett.93.087203
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Besides being an ancient pigment, BaCuSi2O6 is a quasi-2D magnetic insulator with a gapped spin dimer ground state. The application of strong magnetic fields closes this gap, creating a gas of bosonic spin triplet excitations. The topology of the spin lattice makes BaCuSi2O6 an ideal candidate for studying the Bose-Einstein condensation of triplet excitations as a function of the external magnetic field, which acts as a chemical potential. In agreement with quantum Monte Carlo numerical simulations, we observe a distinct lambda anomaly in the specific heat together with a maximum in the magnetic susceptibility upon cooling down to liquid helium temperatures.
引用
收藏
页码:087203 / 1
页数:4
相关论文
共 26 条
[1]   BOSE CONDENSATION IN QUASI-ONE-DIMENSIONAL ANTIFERROMAGNETS IN STRONG FIELDS [J].
AFFLECK, I .
PHYSICAL REVIEW B, 1991, 43 (04) :3215-3222
[2]  
Berke H, 2002, ANGEW CHEM INT EDIT, V41, P2483, DOI 10.1002/1521-3773(20020715)41:14<2483::AID-ANIE2483>3.0.CO
[3]  
2-U
[4]   The National High Magnetic Field Laboratory at Los Alamos National Laboratory [J].
Boebinger, GS ;
Lacerda, AH .
JOURNAL OF LOW TEMPERATURE PHYSICS, 2003, 133 (1-2) :121-138
[5]   Triplet excitations in low-Hc spin-gap systems KCuCl3 and TlCuCl3:: An inelastic neutron scattering study -: art. no. 132415 [J].
Cavadini, N ;
Rüegg, C ;
Furrer, A ;
Güdel, HU ;
Krämer, K ;
Mutka, H ;
Vorderwisch, P .
PHYSICAL REVIEW B, 2002, 65 (13) :1-4
[6]  
FINGER LW, 1989, AM MINERAL, V74, P952
[7]  
FitzHugh E.W., 1992, Studies in conservation, V37, P145, DOI DOI 10.1179/SIC.1992.37.S1.031
[8]   Magnetic phase diagram and structure of the magnetic phases in the quasi-one-dimensional antiferromagnet BaCu2Si2O7:: A symmetry analysis -: art. no. 212405 [J].
Glazkov, V ;
von Nidda, HAK .
PHYSICAL REVIEW B, 2004, 69 (21) :212405-1
[9]   Coarse-grained loop algorithms for Monte Carlo simulation of quantum spin systems [J].
Harada, K ;
Kawashima, N .
PHYSICAL REVIEW E, 2002, 66 (05) :12-056705
[10]   Closing the spin gap in the Kondo insulator Ce3Bi4Pt3 at high magnetic fields [J].
Jaime, M ;
Movshovich, R ;
Stewart, GR ;
Beyermann, WP ;
Berisso, MG ;
Hundley, MF ;
Canfield, PC ;
Sarrao, JL .
NATURE, 2000, 405 (6783) :160-163