Impact of the k-linear term on nonlinear optical response of the C-exciton manifold in ZnO

被引:5
作者
Hazu, K [1 ]
Torii, K
Sota, T
Adachi, S
Chichibu, SF
Cantwell, G
Reynolds, DC
Litton, CW
机构
[1] Waseda Univ, Dept Elect Elect & Comp Engn, Shinjuku Ku, Tokyo 1698555, Japan
[2] Hokkaido Univ, Dept Appl Phys, Kita Ku, Sapporo, Hokkaido 0608628, Japan
[3] Univ Tsukuba, Inst Appl Phys, Grad Sch Pure & Appl Sci, Tsukuba, Ibaraki 3058573, Japan
[4] Zn Technol Inc, Res, Brea, CA 92821 USA
[5] AF Res Lab, Mat & Mfg Directorate, Wright Patterson AFB, OH 45433 USA
[6] Waseda Univ, Grad Sch Sci & Engn, Shinjuku Ku, Tokyo, Japan
[7] Japan Sci & Technol Agcy, CREST, Tokyo, Japan
[8] Japan Sci & Technol Agcy, ERATO, NICP, Chiyoda Ku, Tokyo 1020071, Japan
[9] RIKEN, Photodynam Res Ctr, Aoba Ku, Sendai, Miyagi 9800845, Japan
关键词
D O I
10.1063/1.1710727
中图分类号
O59 [应用物理学];
学科分类号
摘要
Time-integrated and spectrally resolved four-wave mixing (FWM) has been applied to study the impact of the k-linear term on nonlinear optical response of the C-exciton manifold in ZnO. From the excitation wavelength dependence of the FWM signal, we have found possible evidence that the mixing of the Gamma(1) and Gamma(5L) states leads to a three-branch excitonic polariton dispersion but the oscillator strength transfer is small. The energy separation between the lower polariton branch and the extra branch due to the k-linear term has been found to be 3.5 meV. In addition, a binding energy of biexcitons consisting of two C excitons of 1.4 meV has been obtained. (C) 2004 American Institute of Physics.
引用
收藏
页码:5498 / 5501
页数:4
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