Effect of the diffusion anisotropy on the nucleation and growth of xenon on Cu(110)

被引:14
作者
Dienwiebel, M
Zeppenfeld, P [1 ]
Einfeld, J
Comsa, G
Picaud, F
Ramseyer, C
Girardet, C
机构
[1] Johannes Kepler Univ Linz, Inst Expt Phys, A-4040 Linz, Austria
[2] FOM, Inst Atom & Mol Phys, NL-1098 SJ Amsterdam, Netherlands
[3] Forschungszentrum Julich, Inst Schicht & Ionentech, D-52425 Julich, Germany
[4] Univ Bonn, Inst Phys & Theoret Chem, D-53115 Bonn, Germany
[5] Univ Franche Comte, Phys Mol Lab, CNRS, UMR 6624,Fac Sci La Bouloie, F-25030 Besancon, France
关键词
adsorption kinetics; atom-solid interactions; copper; growth; Monte Carlo simulations; noble gases; physical adsorption; scanning tunneling microscopy; stepped single crystal surfaces; surface diffusion;
D O I
10.1016/S0039-6028(99)01131-0
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The growth of Xe on the corrugated Cu(110) surface has been investigated using scanning tunneling microscopy. It is shown that the diffusion anisotropy call lead to the stabilization of energetically unfavored structures and growth modes in two dimensions. In the present case the nucleation and growth occurs at [001]-oriented steps at low surface temperature (13 K) whereas at high higher temperatures (40 K) an almost exclusive decoration of the [110] step edges takes place. These results are explained by interaction calculations and Monte Carlo simulations, (C) 2000 Elsevier Science B,V. All rights reserved.
引用
收藏
页码:L113 / L119
页数:7
相关论文
共 14 条
[1]   Molecular adsorption on unrelaxed and relaxed ionic steps. Application to Ar, CO, CO2, and NH3 adsorbed on MgO(001) [J].
Briquez, S ;
Girardet, C ;
Goniakowski, J ;
Noguera, C .
JOURNAL OF CHEMICAL PHYSICS, 1996, 105 (02) :678-685
[2]  
Brune H, 1998, SURF SCI REP, V31, P121, DOI 10.1016/S0167-5729(99)80001-6
[3]   COARSE TIP DISTANCE ADJUSTMENT AND POSITIONER FOR A SCANNING TUNNELING MICROSCOPE [J].
FROHN, J ;
WOLF, JF ;
BESOCKE, K ;
TESKE, M .
REVIEW OF SCIENTIFIC INSTRUMENTS, 1989, 60 (06) :1200-1201
[4]   AN ULTRAHIGH-VACUUM SCANNING TUNNELING MICROSCOPE FOR USE AT VARIABLE-TEMPERATURE FROM 10-K TO 400-K [J].
HORCH, S ;
ZEPPENFELD, P ;
DAVID, R ;
COMSA, G .
REVIEW OF SCIENTIFIC INSTRUMENTS, 1994, 65 (10) :3204-3210
[5]   DEPOSITION, DIFFUSION AND AGGREGATION OF ATOMS ON SURFACES - A MODEL FOR NANOSTRUCTURE GROWTH [J].
JENSEN, P ;
BARABASI, AL ;
LARRALDE, H ;
HAVLIN, S ;
STANLEY, HE .
PHYSICAL REVIEW B, 1994, 50 (20) :15316-15329
[6]   SURFACE-DIFFUSION OF MOLECULES PHYSISORBED ON DIELECTRIC SUBSTRATES [J].
LAKHLIFI, A ;
GIRARDET, C .
JOURNAL OF CHEMICAL PHYSICS, 1991, 94 (01) :688-694
[7]   XE MONOLAYER ADSORPTION ON CU(110) - EXPERIMENTS AND INTERACTION CALCULATIONS [J].
RAMSEYER, C ;
GIRARDET, C ;
ZEPPENFELD, P ;
GOERGE, J ;
BUCHEL, M ;
COMSA, G .
SURFACE SCIENCE, 1994, 313 (03) :251-265
[8]   BUILDING ONE-DIMENSIONAL AND 2-DIMENSIONAL NANOSTRUCTURES BY DIFFUSION-CONTROLLED AGGREGATION AT SURFACES [J].
RODER, H ;
HAHN, E ;
BRUNE, H ;
BUCHER, JP ;
KERN, K .
NATURE, 1993, 366 (6451) :141-143
[9]   TRANSIT-TIME CONCEPTION FOR ION DIFFUSION THROUGH MEMBRANE CHANNELS [J].
SCHRODER, H .
JOURNAL OF CHEMICAL PHYSICS, 1983, 79 (04) :1991-1996
[10]  
TRINGIDIS MC, 1997, NATO ASI SERIES B, V360