Two-photon induced amplified spontaneous emission from needlelike triphenylamine-containing derivative crystals with low threshold

被引:58
作者
Chen, Qi-Dai [2 ]
Fang, Hong-Hua [2 ]
Xu, Bin [1 ]
Yang, Jie [2 ]
Xia, Hong [2 ]
Chen, Fei-Peng [1 ]
Tian, Wen-Jing [1 ]
Sun, Hong-Bo [2 ]
机构
[1] Jilin Univ, State Key Lab Supramol Struct & Mat, Coll Chem, Changchun 130012, Peoples R China
[2] Jilin Univ, State Key Lab Integrated Optoelect, Coll Elect Sci & Engn, Changchun 130012, Peoples R China
关键词
fluorescence; optical frequency conversion; optical pumping; organic compounds; solid lasers; superradiance; two-photon processes; SINGLE-CRYSTALS; GAIN; ABSORPTION;
D O I
10.1063/1.3142383
中图分类号
O59 [应用物理学];
学科分类号
摘要
Two-photon induced amplified spontaneous emission (ASE) characteristics of a needlelike crystal were studied. Under two-photon excitation, the upconverted light emission was confined within the crystal and self-waveguided along the needle axis then radiated from the needle tips. The full width at half maximum of the two-photon excited fluorescence reaches 6.5 nm and ASE threshold is as low as 0.29 mJ pulse(-1) cm(-2) for the N-(4-(4-(4-(diphenylamino)styryl)styryl)phenyl)-N-phenylbenzene amine crystal, comparable with those achieved by single-photon pumping. The needlelike crystal is shown to be a promising candidate for frequency up-converted organic semiconductor microlasers.
引用
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页数:3
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