Toward strong field mode-selective chemistry

被引:151
作者
Weinacht, TC [1 ]
White, JL [1 ]
Bucksbaum, PH [1 ]
机构
[1] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA
关键词
D O I
10.1021/jp991977x
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We demonstrate a new method for coherent control of bond excitation in the strong field regime. We can selectively excite one or more Raman-active modes in a molecular liquid without the need for externally generated coherent sources separated by the Stokes frequency. The method employs excitation with an intense phase-shaped pulse in a learning control loop.
引用
收藏
页码:10166 / 10168
页数:3
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