Cavity ringdown spectroscopy using mid-infrared quantum-cascade lasers

被引:113
作者
Paldus, BA
Harb, CC
Spence, TG
Zare, RN
Gmachl, C
Capasso, F
Sivco, DL
Baillargeon, JN
Hutchinson, AL
Cho, AY
机构
[1] Informed Diagnost Inc, Sunnyvale, CA 94086 USA
[2] Stanford Univ, Dept Chem, Stanford, CA 94305 USA
[3] Bell Labs, Lucent Technol, Murray Hill, NJ 07974 USA
关键词
D O I
10.1364/OL.25.000666
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Cavity ringdown spectra of ammonia at 10 parts in 10(9) by volume (ppbv) and higher concentrations were recorded by use of a 16-mW continuous-wave quantum-casacde distributed-feedback laser at 8.5 mu m whose wavelength was continuously temperature tuned over 15 nm. A sensitivity (noise-equivalent absorbance) of 3.4 x 10(-9) cm(-1) Hz(-1/2) was achieved for ammonia in nitrogen at standard temperature and pressure, which corresponds to a detection limit of 0.25 ppbv. (C) 2000 Optical Society of America.
引用
收藏
页码:666 / 668
页数:3
相关论文
共 13 条
[11]   High-resolution (Doppler-limited) spectroscopy using quantum-cascade distributed-feedback lasers [J].
Sharpe, SW ;
Kelly, JF ;
Hartman, JS ;
Gmachl, C ;
Capasso, F ;
Sivco, DL ;
Baillargeon, JN ;
Cho, AY .
OPTICS LETTERS, 1998, 23 (17) :1396-1398
[12]   A laser-locked cavity ring-down spectrometer employing an analog detection scheme [J].
Spence, TG ;
Harb, CC ;
Paldus, BA ;
Zare, RN ;
Willke, B ;
Byer, RL .
REVIEW OF SCIENTIFIC INSTRUMENTS, 2000, 71 (02) :347-353
[13]   Kilohertz linewidth from frequency-stabilized mid-infrared quantum cascade lasers [J].
Williams, RM ;
Kelly, JF ;
Hartman, JS ;
Sharpe, SW ;
Taubman, MS ;
Hall, JL ;
Capasso, F ;
Gmachl, C ;
Sivco, DL ;
Baillargeon, JN ;
Cho, AY .
OPTICS LETTERS, 1999, 24 (24) :1844-1846