Optical pump-probe spectroscopy with 7-fs pump pulses and a probe spectrum wider than 0.7 eV reveals the ultrafast carrier dynamics in freestanding thin graphite films. We discern for the first time a rapid intraband carrier equilibration within 30 fs, leaving the system with separated electron and hole chemical potentials. Phonon-mediated intraband cooling of electrons and holes occurs on a 100 fs time scale. The kinetics are in agreement with simulations based on Boltzmann equations.
机构:
Univ Manchester, Manchester Ctr Mesosci & Nanotechnol, Manchester M13 9PL, Lancs, EnglandUniv Manchester, Manchester Ctr Mesosci & Nanotechnol, Manchester M13 9PL, Lancs, England
Geim, A. K.
;
Novoselov, K. S.
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Univ Manchester, Manchester Ctr Mesosci & Nanotechnol, Manchester M13 9PL, Lancs, EnglandUniv Manchester, Manchester Ctr Mesosci & Nanotechnol, Manchester M13 9PL, Lancs, England
机构:
Donostia Int Phys Ctr, San Sebastian 20018, Spain
Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USANatl Inst Mat Sci, Adv Nanocharacterizat Ctr, Tsukuba, Ibaraki 3050047, Japan
机构:
Univ Manchester, Manchester Ctr Mesosci & Nanotechnol, Manchester M13 9PL, Lancs, EnglandUniv Manchester, Manchester Ctr Mesosci & Nanotechnol, Manchester M13 9PL, Lancs, England
Geim, A. K.
;
Novoselov, K. S.
论文数: 0引用数: 0
h-index: 0
机构:
Univ Manchester, Manchester Ctr Mesosci & Nanotechnol, Manchester M13 9PL, Lancs, EnglandUniv Manchester, Manchester Ctr Mesosci & Nanotechnol, Manchester M13 9PL, Lancs, England
机构:
Donostia Int Phys Ctr, San Sebastian 20018, Spain
Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USANatl Inst Mat Sci, Adv Nanocharacterizat Ctr, Tsukuba, Ibaraki 3050047, Japan