Ultrafast Carrier Dynamics in Graphite

被引:397
作者
Breusing, Markus [1 ]
Ropers, Claus [1 ,2 ]
Elsaesser, Thomas [1 ]
机构
[1] Max Born Inst Nichtlineare Opt & Kurzzeitspektros, D-12489 Berlin, Germany
[2] Univ Gottingen, Courant Res Ctr Nanospect & Xray Imaging, D-3400 Gottingen, Germany
关键词
GRAPHENE;
D O I
10.1103/PhysRevLett.102.086809
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Optical pump-probe spectroscopy with 7-fs pump pulses and a probe spectrum wider than 0.7 eV reveals the ultrafast carrier dynamics in freestanding thin graphite films. We discern for the first time a rapid intraband carrier equilibration within 30 fs, leaving the system with separated electron and hole chemical potentials. Phonon-mediated intraband cooling of electrons and holes occurs on a 100 fs time scale. The kinetics are in agreement with simulations based on Boltzmann equations.
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页数:4
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