Photoluminescence spectroscopy of single CdSe nanocrystallite quantum dots

被引:641
作者
Empedocles, SA
Norris, DJ
Bawendi, MG
机构
[1] Massachusetts Institute of Technology, Cambridge, MA
关键词
D O I
10.1103/PhysRevLett.77.3873
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We collect and spectrally resolve photoluminescence from single CdSe nanocrystallite quantum dots. The elimination of spectral inhomogeneities reveals resolution limited spectral linewidths (<120 mu eV at 10 K) more than 50 times narrower than expected from ensemble measurements. Light driven spectral diffusion is observed as a form of power broadening. These studies confirm the atomiclike nature of the emitting state in CdSe nanocrystallites.
引用
收藏
页码:3873 / 3876
页数:4
相关论文
共 29 条
[1]   ELECTRON-VIBRATION COUPLING IN SEMICONDUCTOR CLUSTERS STUDIED BY RESONANCE RAMAN-SPECTROSCOPY [J].
ALIVISATOS, AP ;
HARRIS, TD ;
CARROLL, PJ ;
STEIGERWALD, ML ;
BRUS, LE .
JOURNAL OF CHEMICAL PHYSICS, 1989, 90 (07) :3463-3468
[2]   Semiconductor clusters, nanocrystals, and quantum dots [J].
Alivisatos, AP .
SCIENCE, 1996, 271 (5251) :933-937
[3]  
BASCHE T, IN PRESS
[4]   SINGLE MOLECULES OBSERVED BY NEAR-FIELD SCANNING OPTICAL MICROSCOPY [J].
BETZIG, E ;
CHICHESTER, RJ .
SCIENCE, 1993, 262 (5138) :1422-1425
[5]   PHOTOLUMINESCENCE OF SINGLE SEMICONDUCTOR NANOCRYSTALLITES BY 2-PHOTON EXCITATION MICROSCOPY [J].
BLANTON, SA ;
DEHESTANI, A ;
LIN, PC ;
GUYOTSIONNEST, P .
CHEMICAL PHYSICS LETTERS, 1994, 229 (03) :317-322
[6]   SHARP-LINE PHOTOLUMINESCENCE OF EXCITONS LOCALIZED AT GAAS/ALGAAS QUANTUM-WELL INHOMOGENEITIES [J].
BRUNNER, K ;
ABSTREITER, G ;
BOHM, G ;
TRANKLE, G ;
WEIMANN, G .
APPLIED PHYSICS LETTERS, 1994, 64 (24) :3320-3322
[7]   QUANTUM CRYSTALLITES AND NONLINEAR OPTICS [J].
BRUS, L .
APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING, 1991, 53 (06) :465-474
[9]  
DABBOUSI BO, IN PRESS
[10]   PREPARATION OF II-VI QUANTUM-DOT COMPOSITES BY ELECTROSPRAY ORGANOMETALLIC CHEMICAL-VAPOR-DEPOSITION [J].
DANEK, M ;
JENSEN, KF ;
MURRAY, CB ;
BAWENDI, MG .
JOURNAL OF CRYSTAL GROWTH, 1994, 145 (1-4) :714-720