Methane oxidation in a dielectric barrier discharge. The impact of discharge power and discharge gap filling

被引:5
作者
Khassin, AA [1 ]
Pietruszka, BL
Heintze, M
Parmon, VN
机构
[1] Boreskov Inst Catalysis, Novosibirsk 630090, Russia
[2] Inst Low Temp Plasma Phys, D-17489 Greifswald, Germany
来源
REACTION KINETICS AND CATALYSIS LETTERS | 2004年 / 82卷 / 01期
关键词
dielectric barrier discharge; methane oxidation; plasma-induced reaction; catalysis; surface;
D O I
10.1023/B:REAC.0000028812.77120.f9
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The conversion of an air-methane mixture in a dielectric barrier discharge (DBD) was studied in a wide range of temperatures and discharge powers for different gap fillings. The impact of the gap filling surface area appears to be negligible at temperatures below 530 K, while being significant above 570 K. Some processes on the surface are countercurrent to those in the DBD plasma.
引用
收藏
页码:111 / 119
页数:9
相关论文
共 15 条
[1]  
Cormier JM, 2002, HIGH TEMP MATER P-US, V6, P421
[2]   NONEQUILIBRIUM VOLUME PLASMA CHEMICAL-PROCESSING [J].
ELIASSON, B ;
KOGELSCHATZ, U .
IEEE TRANSACTIONS ON PLASMA SCIENCE, 1991, 19 (06) :1063-1077
[3]  
EREMIN EN, 1968, ELEMENTS GAS ELECTRO
[4]  
HEINTZE M, 2003, IN PRESS CATAL TODAY
[5]   CO2 reforming of CH4 by atmospheric pressure ac discharge plasmas [J].
Huang, AM ;
Xia, GG ;
Wang, JY ;
Suib, SL ;
Hayashi, Y ;
Matsumoto, H .
JOURNAL OF CATALYSIS, 2000, 189 (02) :349-359
[6]   Characterization of the nickel-amesite-chlorite-vermiculite system. Part I. Silicon binding in Ni-Mg-Al phylloaluminosilicates [J].
Khassin, AA ;
Yurieva, TM ;
Demeshkina, MP ;
Kustova, GN ;
Itenberg, IS ;
Kaichev, VV ;
Plyasova, LM ;
Anufrienko, VF ;
Molina, IY ;
Larina, TV ;
Baronskaya, NA ;
Parmon, VN .
PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2003, 5 (18) :4025-4031
[7]   CO2 reforming of methane by the combination of dielectric-barrier discharges and catalysis [J].
Kraus, M ;
Eliasson, B ;
Kogelschatz, U ;
Wokaun, A .
PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2001, 3 (03) :294-300
[8]  
PIETRUSZKA B, UNPUB APPL CATAL B
[9]   On a possible mechanism of the methane steam reforming in a gliding arc reactor [J].
Rusu, I ;
Cormier, JM .
CHEMICAL ENGINEERING JOURNAL, 2003, 91 (01) :23-31
[10]   Chemical quasi-equilibria: a new concept in the description of reactive plasmas [J].
Rutscher, A. ;
Wagner, H-E .
PLASMA SOURCES SCIENCE & TECHNOLOGY, 1993, 2 (04) :279-288