Multifunctional, multilayer, multiscale:: Integrative synthesis of complex macroporous and mesoporous thin films with spatial separation of porosity and function

被引:74
作者
Angelome, Paula C. [1 ]
Fuertes, M. Cecilia [1 ]
Soler-Illia, Galo J. A. A. [1 ]
机构
[1] Comis Nacl Energma Atom, Ctr Atom Constituyentes, Unidad Activ Quim, Buenos Aires, DF, Argentina
关键词
D O I
10.1002/adma.200600439
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Complex multilayered thin-film architectures are fabricated by sequentially stacking mesoporous and macroporous layers with varying structure and properties. A series of deposition-stabilization steps are used to sequentially deposit the component layers of the films in order to obtain interconnected systems with a precise ordering of accessible cavities, as shown in the figure.
引用
收藏
页码:2397 / +
页数:7
相关论文
共 45 条
[1]   Ag/AgCl-loaded ordered mesoporous anatase for photocatalysis [J].
Andersson, M ;
Birkedal, H ;
Franklin, NR ;
Ostomel, T ;
Boettcher, S ;
Palmqvist, AEC ;
Stucky, GD .
CHEMISTRY OF MATERIALS, 2005, 17 (06) :1409-1415
[2]   Ordered mesoporous hybrid thin films with double organic functionality and mixed oxide framework [J].
Angelomé, PC ;
Soler-Illia, GJDA .
JOURNAL OF MATERIALS CHEMISTRY, 2005, 15 (35-36) :3903-3912
[3]   Hybrid non-silica mesoporous thin films [J].
Angelomé, PC ;
Aldabe-Bilmes, S ;
Calvo, ME ;
Crepaldi, EL ;
Grosso, D ;
Sanchez, C ;
Soler-Illia, GJAA .
NEW JOURNAL OF CHEMISTRY, 2005, 29 (01) :59-63
[4]   Organically modified transition-metal oxide mesoporous thin films and xerogels [J].
Angelomé, PC ;
Soler-Illia, GJDAA .
CHEMISTRY OF MATERIALS, 2005, 17 (02) :322-331
[5]   Promises and problems of mesoscale materials chemistry or why meso? [J].
Antonietti, M ;
Ozin, GA .
CHEMISTRY-A EUROPEAN JOURNAL, 2004, 10 (01) :28-41
[6]   LIQUID-CRYSTALLINE PHASES AS TEMPLATES FOR THE SYNTHESIS OF MESOPOROUS SILICA [J].
ATTARD, GS ;
GLYDE, JC ;
GOLTNER, CG .
NATURE, 1995, 378 (6555) :366-368
[7]   One-step template-directed synthesis of multifunctionalised nanoporous silica:: on the way to interactive nanomaterials [J].
Besson, E ;
Mehdi, A ;
Matsura, V ;
Guari, Y ;
Reyé, C ;
Corriu, RJP .
CHEMICAL COMMUNICATIONS, 2005, (13) :1775-1777
[8]   Phase diagram for mesoporous CTAB-silica films prepared under dynamic conditions [J].
Besson, S ;
Gacoin, T ;
Ricolleau, C ;
Jacquiod, C ;
Boilot, JP .
JOURNAL OF MATERIALS CHEMISTRY, 2003, 13 (02) :404-409
[9]   Silver nanoparticle growth in 3D-hexagonal mesoporous silica films [J].
Besson, S ;
Gacoin, T ;
Ricolleau, C ;
Boilot, JP .
CHEMICAL COMMUNICATIONS, 2003, (03) :360-361
[10]   Nanotectonic approach of the texturation of CeO2 based nanomaterials [J].
Bouchara, A ;
Soler-Illia, GJDA ;
Chane-Ching, JY ;
Sanchez, C .
CHEMICAL COMMUNICATIONS, 2002, (11) :1234-1235