Balsa Raft Crossing the Pacific Finds Low Contaminant Levels

被引:39
作者
Goksoyr, Anders [1 ,2 ]
Tollefsen, Knut Erik [3 ,4 ]
Grung, Merete [3 ]
Loken, Katharina [5 ]
Lie, Elisabeth [5 ]
Zenker, Armin [6 ]
Fent, Karl [6 ,7 ]
Schlabach, Martin [8 ]
Huber, Sandra [9 ]
机构
[1] Univ Bergen, Dept Mol Biol, N-5020 Bergen, Norway
[2] Biosense Labs AS, N-5008 Bergen, Norway
[3] Norwegian Inst Water Res NIVA, N-0349 Oslo, Norway
[4] Univ Life Sci, Dept Plant & Environm Sci, N-1432 As, Norway
[5] Norwegian Sch Vet Sci, N-0033 Oslo, Norway
[6] Univ Appl Sci NW Switzerland, CH-4132 Muttenz, Switzerland
[7] Swiss Fed Inst Technol, Zurich, Switzerland
[8] Norwegian Inst Air Res NILU, N-2027 Kjeller, Norway
[9] Polar Environm Ctr, Norwegian Inst Air Res NILU, N-9296 Tromso, Norway
关键词
SEMIPERMEABLE-MEMBRANE DEVICES; POLYBROMINATED DIPHENYL ETHERS; SEA-SURFACE MICROLAYER; FLAME RETARDANTS; UV FILTERS; PERFLUORINATED ACIDS; NORTH PACIFIC; WASTE-WATER; SPMDS; POLLUTANTS;
D O I
10.1021/es900154h
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
During the Norwegian Tangaroa balsa raft expedition crossing the Pacific in 2006, surface water samples were collected by passive semipermeable membrane device (SPMD) sampling, active surface microlayer collection, and fish bile collection. The samples were analyzed for water contamination including a range of persistent organochlorine contaminants, pesticides, polycyclic aromatic hydrocarbons, as well as modern widespread chemicals such as brominated flame retardants, UV-filters, and perfluorinated compounds, using a network of expert laboratories and advanced instrumentation. Only trace to undetectable levels of all compounds were observed in both SPMDs and microlayer samples. The data from SPMDs were used to estimate surface water concentrations by back-calculation using sampling rates published in the literature. Conservative factors indicate that the levels in the surface waters are in the pg/L to subpg/L range for organochlorines, BFRs, and PFCs, indicating the central Pacific Ocean stil! represents a pristine environment for oceanic life.
引用
收藏
页码:4783 / 4790
页数:8
相关论文
共 40 条
[1]  
AAS E, 2006, BIOL EFFECTS CONTAMI
[2]   Longitudinal and Latitudinal Distribution of Perfluoroalkyl Compounds in the Surface Water of the Atlantic Ocean [J].
Ahrens, Lutz ;
Barber, Jonathan L. ;
Xie, Zhiyong ;
Ebinghaus, Ralf .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2009, 43 (09) :3122-3127
[3]   Occurrence of some organic UV filters in wastewater, in surface waters, and in fish from Swiss lakes [J].
Balmer, ME ;
Buser, HR ;
Müller, MD ;
Poiger, T .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2005, 39 (04) :953-962
[4]   Validation of a screening method based on liquid chromatography coupled to high-resolution mass spectrometry for analysis of perfluoroalkylated substances in biota [J].
Berger, U ;
Haukås, M .
JOURNAL OF CHROMATOGRAPHY A, 2005, 1081 (02) :210-217
[5]   Do flame retardants threaten ocean life? [J].
de Boer, J ;
Wester, PG ;
Klammer, HJC ;
Lewis, WE ;
Boon, JP .
NATURE, 1998, 394 (6688) :28-29
[6]   Diffuse pollution of surface water by pharmaceutical products [J].
Derksen, JGM ;
Rijs, GBJ ;
Jongbloed, RH .
WATER SCIENCE AND TECHNOLOGY, 2004, 49 (03) :213-221
[7]   PHOTOPROTECTION OF WOOL BY APPLICATION OF ULTRAVIOLET ABSORBER-POLYMER MIXTURES TO ITS SURFACE [J].
EVANS, NA ;
WATERS, PJ .
TEXTILE RESEARCH JOURNAL, 1981, 51 (06) :432-434
[8]   Monitoring of organotin compounds in seawater using semipermeable membrane devices (SPMDs) - tentative results [J].
Folsvik, N ;
Brevik, EM ;
Berge, JA .
JOURNAL OF ENVIRONMENTAL MONITORING, 2000, 2 (04) :281-284
[9]   Riverine inputs of polybrominated diphenyl ethers from the Pearl River Delta (China) to the coastal ocean [J].
Guan, Yu-Feng ;
Wang, Ji-Zhong ;
Ni, Hong-Gang ;
Luo, Xiao-Jun ;
Mai, Bi-Xian ;
Zeng, Eddy Y. .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2007, 41 (17) :6007-6013
[10]   Uptake rates of alkylphenols, PAHs and carbazoles in semipermeable membrane devices (SPMDs) and polar organic chemical integrative samplers (POCIS) [J].
Harman, C. ;
Tollefsen, K-E. ;
Boyum, O. ;
Thomas, K. ;
Grung, M. .
CHEMOSPHERE, 2008, 72 (10) :1510-1516